ULTRAFAST NONLINEAR SPECTROSCOPY WITH CHIRPED OPTICAL PULSES

被引：97

作者：

NIBBERING, ETJ ^{[1
]}

WIERSMA, DA ^{[1
]}

DUPPEN, K ^{[1
]}

机构：

[1] UNIV GRONINGEN,CTR MAT SCI,9747 AG GRONINGEN,NETHERLANDS

来源：

PHYSICAL REVIEW LETTERS | 1992年 / 68卷 / 04期

关键词：

D O I：

10.1103/PhysRevLett.68.514

中图分类号：

O4 [物理学];

学科分类号：

0702 ;

摘要：

Ultrafast four-wave mixing experiments using chirped-pulse excitation of a dye molecule in solution are reported and analyzed. Novel time-delayed signals are observed which are assigned to coherent Stokes-Raman scattering involving the excited state. Numerical calculations of four-wave mixing with linearly chirped pulses based on a stochastic dynamical model show that the signal near zero delay time is extremely sensitive to the presence or absence of slow fluctuations in the solute-solvent interaction.

引用

页码：514 / 517

页数：4

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