ULTRAFAST NONLINEAR SPECTROSCOPY WITH CHIRPED OPTICAL PULSES

被引：97

作者：

NIBBERING, ETJ ^{[1
]}

WIERSMA, DA ^{[1
]}

DUPPEN, K ^{[1
]}

机构：

[1] UNIV GRONINGEN,CTR MAT SCI,9747 AG GRONINGEN,NETHERLANDS

来源：

PHYSICAL REVIEW LETTERS | 1992年 / 68卷 / 04期

关键词：

D O I：

10.1103/PhysRevLett.68.514

中图分类号：

O4 [物理学];

学科分类号：

0702 ;

摘要：

Ultrafast four-wave mixing experiments using chirped-pulse excitation of a dye molecule in solution are reported and analyzed. Novel time-delayed signals are observed which are assigned to coherent Stokes-Raman scattering involving the excited state. Numerical calculations of four-wave mixing with linearly chirped pulses based on a stochastic dynamical model show that the signal near zero delay time is extremely sensitive to the presence or absence of slow fluctuations in the solute-solvent interaction.

引用

页码：514 / 517

页数：4

共 12 条

[1] FEMTOSECOND PHOTON-ECHOES FROM MOLECULES IN SOLUTION
BECKER, PC
FRAGNITO, HL
BIGOT, JY
CRUZ, CHB
FORK, RL
SHANK, CV
[J]. PHYSICAL REVIEW LETTERS, 1989, 63 (05) : 505 - 507
[2] NON-MARKOVIAN DEPHASING OF MOLECULES IN SOLUTION MEASURED WITH 3-PULSE FEMTOSECOND PHOTON-ECHOES
BIGOT, JY
PORTELLA, MT
SCHOENLEIN, RW
BARDEEN, CJ
MIGUS, A
SHANK, CV
[J]. PHYSICAL REVIEW LETTERS, 1991, 66 (09) : 1138 - 1141
[3] FAINBERG BD, 1983, OPT SPEKTROSK+, V55, P1098
[4] COMPRESSION OF OPTICAL PULSES TO 6 FEMTOSECONDS BY USING CUBIC PHASE COMPENSATION
FORK, RL
CRUZ, CHB
BECKER, PC
SHANK, CV
[J]. OPTICS LETTERS, 1987, 12 (07) : 483 - 485
[5] KUBO R, 2007, ADV CHEM PHYS, P101, DOI DOI 10.1002/9780470143605.CH6
[6] NONLINEAR RESPONSE FUNCTION FOR TIME-DOMAIN AND FREQUENCY-DOMAIN 4-WAVE-MIXING
MUKAMEL, S
LORING, RF
[J]. JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 1986, 3 (04) : 595 - 606
[7] NAKATSUKA H, 1981, PHYS REV LETT, V47, P910, DOI 10.1103/PhysRevLett.47.910
[8] FEMTOSECOND NON-MARKOVIAN OPTICAL-DYNAMICS IN SOLUTION
NIBBERING, ETJ
WIERSMA, DA
DUPPEN, K
[J]. PHYSICAL REVIEW LETTERS, 1991, 66 (19) : 2464 - 2467
[9] NIBBERING ETJ, IN PRESS
[10] APPLICATION OF CHIRPED PULSES TO THE MEASUREMENT OF ULTRASHORT PHASE RELAXATION-TIME IN A SEMICONDUCTOR-DOPED GLASS
TOKIZAKI, T
ISHIDA, Y
YAJIMA, T
[J]. OPTICS COMMUNICATIONS, 1989, 71 (06) : 355 - 358

← 1 2 →