RELAXATIONAL AND VIBRATIONAL CONTRIBUTIONS TO THE DYNAMICS OF THE GLASS-TRANSITION

被引:17
作者
SOKOLOV, AP [1 ]
ROSSLER, E [1 ]
KISLIUK, A [1 ]
SOLTWISCH, M [1 ]
QUITMANN, D [1 ]
机构
[1] RUSSIAN ACAD SCI,INST AUTOMAT & ELECTROMETRY,NOVOSIBIRSK 630090,RUSSIA
来源
PHYSICA A | 1993年 / 201卷 / 1-3期
关键词
D O I
10.1016/0378-4371(93)90400-X
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The low-frequency Raman spectra of a few glass forming liquids were analysed. It is shown that the main difference of the spectra for strong and fragile glass formers is the ratio of vibrational to relaxation contributions: the stronger the glass former, the higher is the vibrational contribution. It is shown that this difference correlates with the difference in the low-temperature anomalies of glasses. The spectra are compared with the mode coupling theory predictions. Qualitatively the predicted behavior is observed in all cases, however, some quantitative disagreement is found.
引用
收藏
页码:67 / 71
页数:5
相关论文
共 10 条
  • [1] Angell C. A, 1984, RELAXATIONS COMPLEX, P3
  • [2] H-BOND DYNAMICS IN WELL-CHARACTERIZED SUPERCOOLED AND GLASSY AQUEOUS-SOLUTIONS
    DUPUY, J
    JAL, JF
    CHIEUX, P
    [J]. JOURNAL OF MOLECULAR STRUCTURE, 1991, 250 (2-4) : 315 - 328
  • [3] FAST LOCAL MOTION AROUND TG IN A MOLECULAR GLASS AS OBSERVED BY INCOHERENT NEUTRON-SCATTERING
    FUJARA, F
    PETRY, W
    [J]. EUROPHYSICS LETTERS, 1987, 4 (08): : 921 - 927
  • [4] SECONDARY RELAXATION IN THE GLASS-TRANSITION REGIME OF ORTHO-TERPHENYL OBSERVED BY INCOHERENT NEUTRON-SCATTERING
    KIEBEL, M
    BARTSCH, E
    DEBUS, O
    FUJARA, F
    PETRY, W
    SILLESCU, H
    [J]. PHYSICAL REVIEW B, 1992, 45 (18): : 10301 - 10305
  • [5] TESTING MODE-COUPLING PREDICTIONS FOR ALPHA-RELAXATION AND BETA-RELAXATION IN CA0.4K0.6(NO3)1.4 NEAR THE LIQUID-GLASS TRANSITION BY LIGHT-SCATTERING
    LI, G
    DU, WM
    CHEN, XK
    CUMMINS, HZ
    TAO, NJ
    [J]. PHYSICAL REVIEW A, 1992, 45 (06): : 3867 - 3879
  • [6] Phillips W. A., 1981, AMORPHOUS SOLIDS
  • [7] LOW-ENERGY ANOMALIES OF VIBRATIONAL-SPECTRA AND MEDIUM-RANGE ORDER IN GLASSES
    SOKOLOV, AP
    KISLIUK, A
    SOLTWISCH, M
    QUITMANN, D
    [J]. PHYSICA A, 1993, 201 (1-3): : 295 - 299
  • [8] SOKOLOV AP, IN PRESS
  • [9] WHITE GK, 1977, J NONCRYST SOLIDS, V23, P99
  • [10] [No title captured]