OPTICAL HETERODYNE-DETECTION OF IMPULSIVE STIMULATED RAMAN-SCATTERING IN LIQUIDS

被引：58

作者：

CHANG, YJ

CONG, P

SIMON, JD

机构：

[1] UNIV CALIF SAN DIEGO,DEPT CHEM & BIOCHEM,LA JOLLA,CA 92093

[2] UNIV CALIF SAN DIEGO,INST NONLINEAR SCI,LA JOLLA,CA 92093

来源：

JOURNAL OF PHYSICAL CHEMISTRY | 1995年 / 99卷 / 20期

关键词：

D O I：

10.1021/j100020a004

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Optical heterodyne detection is implemented in an impulsive stimulated Raman scattering (ISRS) experiment by the use of a Mach-Zehnder interferometer. The combination of polarization-selective ISRS and heterodyne detection allows direct measurements of the real and imaginary parts of an arbitrary element of the third-rank material response tenser chi((3)). The heterodyne-detected chi(1111)((3))(t) of CS2 is presented and compared with the homodyne-detected response.

引用

页码：7857 / 7859

页数：3

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