Radiometric methods were used to investigate the radioactive properties of rocks in parts of southwestern Nigeria with a view to interpreting the geological structure and abundance of natural radioactive elements in the main type rocks. The airborne radiometric dataset of Ikole Sheet and ground radiometric data recorded from eight traverses in Akoko axis of the study area were processed. Results presented as maps and profiles displayed variations of high and low radioactive concentrations across the area. These maps showed moderate to very high concentrations and very low to low concentrations of the radioelements; uranium (4.5-13.0 ppm); (LLD-low limit of detection -3.0 ppm), Th (25.0-70.0 ppm); (8.5-16.0 ppm) and K (2.0-4.0 %); but the most often observed values are in the range 2.5-7.0 ppm, 22.0-30.0 ppm and 3.0-4.0% for U, Th, and K respectively. High concentrations imply that the rocks are crystalline, undeformed and are rich in feldspar and U-Th bearing minerals. While low radioactivity is attributed to varying geologic framework compositions, weathered materials or fluids formed as a result of intense metamorphism. The radiometric datasets proved valuable in delineating different rock types and serve as a complementary tool in identifying geochemical zoning of rocks in the area. (c) 2018 Vietnam Academy of Science and Technology