AMPLIFIED SPONTANEOUS EMISSION OVER THE XEF(D-]X) TRANSITION IN SOLID KR

被引:12
作者
KUNTTU, H
LAWRENCE, WG
APKARIAN, VA
机构
[1] Department of Chemistry, Institute for Surface and Interface Science, University of California, Irvine
关键词
D O I
10.1063/1.459940
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
XeF doped solid Kr represents a novel solid state exciplex laser. A net gain in excess of 100 cm-1 and a superradiant beam of 5 mrad divergence are observed over the XeF(D --> X) transition at 301 nm, when free standing crystals of XeF doped Kr are optically pumped near the XeF(D <-- X) absorption maximum at 260 nm. Superlinear dependence of gain on pump intensity and low divergence of the amplified beam are taken as evidence for self-focusing. The XeF (D) state is effectively isolated from the lower manifold of charge transfer states in solid Kr, which includes XeF(B,C) and (KrXe) +F-.
引用
收藏
页码:1692 / 1697
页数:6
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