Evaluation on the removal efficiency of pharmaceutical compounds in conventional drinking water treatment processes

被引:1
作者
Seo, Hee-Jeong [1 ]
Park, Yong-Hoon [1 ]
Kang, In-Sook [1 ]
Myong, Hwa-Bong [1 ]
Song, Yang-Suk [1 ]
Kang, Yeong-Ju [1 ]
机构
[1] Water Qual Res Inst Waterworks Gwangju, Gwangju, South Korea
关键词
pharmaceutical compound; antibiotics; adsorption; coagulation;
D O I
10.5806/AST.2016.29.3.126
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
In the present study, we evaluated the efficiency of the drinking water treatment unit processes controlled by targeting high pharmaceutical compounds that are likely to be released into the water supply. In the coagulation process, the removal rate of sulfonamide, an antibiotic, amounted to 22.6 similar to 42.1 %, that of naproxen to 28.2 %, and that of acetaminophen to 20 %. Trimethoprim has demonstrated a low removal rate (4.4 %), while the removal rate of erythromycin was 2.4 %; aspirin was not removed at all. When applying a mixture of chlorination and the coagulation process, the removal rate was increased with increasing the chlorine dosage. When the chlorine injection with the concentration of 3 mg/L was applied, sulfonamide antibiotics, acetaminophen and naproxen, were completely removed. Trimethoprim exhibited a high removal efficiency of ca. 98%, while the removal efficiency of erythromycin was about 55 %; at the same time, aspirin showed a lower removal ratio (ca. 10 %). When applying the powdered activated carbon adsorption process, the removal rate was increased with increase of the concentration of the powder activated carbon injection. Sulfonamide antibiotics showed about 18 similar to 50 % removal efficiency in the 1 mg/L, the removal rate was increased by at least 80 % in 25 mg/L. The evaluation results of the titration injection concentration of chlorine treatment and adsorption, coagulation process for the efficient processing of the remaining pharmaceutical compounds in the water treatment process, when applying the chlorine 3 mg/L, powdered activated carbon 10 mg/L and coagulant 15 mg/L were removed more than 90 %.
引用
收藏
页码:126 / 135
页数:10
相关论文
共 15 条
[1]   Removal of antibiotics from surface and distilled water in conventional water treatment processes [J].
Adams, C ;
Wang, Y ;
Loftin, K ;
Meyer, M .
JOURNAL OF ENVIRONMENTAL ENGINEERING-ASCE, 2002, 128 (03) :253-260
[2]   Antibiotics and antibiotic resistance in water environments [J].
Baquero, Fernando ;
Martinez, Jose-Luis ;
Canton, Rafael .
CURRENT OPINION IN BIOTECHNOLOGY, 2008, 19 (03) :260-265
[3]  
김주형, 2008, [JOURNAL OF ENVIRONMENTAL ANALYSIS, HEALTH AND TOXICOLOGY, 환경분석과 독성보건], V11, P109
[4]  
Ministry of Food and Drug Safety, 2015, 2015 FOOD DRUG STAT
[5]  
National Institute of Environmental Research, 2010, PHARM ENV SORC FAT 3
[6]  
National Institute of Environmental Research, 2007, DEV AN METH STUD EXP
[7]  
Son H. -J., 2011, J KOR SOC ENV ENG, V33, P453
[8]   Efficiency of conventional drinking-water-treatment processes in removal of pharmaceuticals and other organic compounds [J].
Stackelberg, Paul E. ;
Gibs, Jacob ;
Furlong, Edward T. ;
Meyer, Michael T. ;
Zaugg, Steven D. ;
Lippincott, R. Lee .
SCIENCE OF THE TOTAL ENVIRONMENT, 2007, 377 (2-3) :255-272
[9]   Persistence of pharmaceutical compounds and other organic wastewater contaminants in a conventional drinking-watertreatment plant [J].
Stackelberg, PE ;
Furlong, ET ;
Meyer, MT ;
Zaugg, SD ;
Henderson, AK ;
Reissman, DB .
SCIENCE OF THE TOTAL ENVIRONMENT, 2004, 329 (1-3) :99-113
[10]   Removal of pharmaceuticals during drinking water treatment [J].
Ternes, TA ;
Meisenheimer, M ;
McDowell, D ;
Sacher, F ;
Brauch, HJ ;
Gulde, BH ;
Preuss, G ;
Wilme, U ;
Seibert, NZ .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2002, 36 (17) :3855-3863