THE EFFECT OF FIXED-BED REACTOR CONFIGURATION ON THE OXIDATIVE COUPLING OF METHANE OVER A LI/PB/CA CATALYST

被引：16

作者：

SMITH, KJ

PAINTER, TM

GALUSZKA, J

机构：

[1] ALBERTA RES COUNCIL,DEPT COAL & HYDROCARBON PROC,DEVON T0C 1E0,ALBERTA,CANADA

[2] CANADA CTR MINERAL & ENERGY TECHNOL,ENERGY RES LABS,OTTAWA K1A OG1,ONTARIO,CANADA

来源：

CATALYSIS LETTERS | 1991年 / 11卷 / 3-6期

关键词：

METHANE; OXIDATIVE COUPLING; CATALYST; REACTOR CONFIGURATION;

D O I：

10.1007/BF00764321

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Introduction of additional O2 at the midpoint of the catalyst bed of a methane oxidative coupling, fixed bed reactor, increases the C2 STY more than the COx STY over a Li/Pb/Ca catalyst. This observation is not only a consequence of kinetics but may also be attributed to increased methyl radical generation on the O2 replenished catalyst surface.

引用

页码：301 / 307

页数：7

共 50 条

[1] Model-Based Catalyst Selection for the Oxidative Coupling of Methane in an Adiabatic Fixed-Bed Reactor
Pirro, Laura
Obradovic, Ana
Vandegehuchte, Bart D.
Marin, Guy B.
Thybaut, Joris W.
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2018, 57 (48) : 16295 - 16307
[2] Reaction engineering studies in a polytropic fixed-bed reactor over a highly active and selective catalyst for oxidative methane coupling
Mleczko, Leslaw
Gayko, Guido
Niemi, Vesa M.
Hiltunen, Jyrki
Chemical Engineering and Technology, 1997, 20 (01): : 29 - 35
[3] Reaction engineering studies in a polytropic fixed-bed reactor over a highly active and selective catalyst for oxidative methane coupling
Mleczko, L
Gayko, G
Niemi, VM
Hiltunen, J
CHEMICAL ENGINEERING & TECHNOLOGY, 1997, 20 (01) : 29 - 35
[4] Numerical simulation of fixed bed reactor for oxidative coupling of methane over monolithic catalyst
Zhang, Zhao
Guo, Ziqi
Ji, Shengfu
CHINESE JOURNAL OF CHEMICAL ENGINEERING, 2015, 23 (10) : 1627 - 1633
[5] Catalytic Decomposition of 2% Methanol in Methane over Metallic Catalyst by Fixed-Bed Catalytic Reactor
Awad, Ali
Ahmed, Israr
Qadir, Danial
Khan, Muhammad Saad
Idris, Alamin
ENERGIES, 2021, 14 (08)
[6] Oxidative coupling of methane in a fixed bed reactor over perovskite catalyst:A simulation study using experimental kinetic model
Nakisa Yaghobi
Mir Hamid Reza Ghoreishy
Journal of Natural Gas Chemistry, 2008, (01) : 8 - 16
[7] Oxidative coupling of methane in a fixed bed reactor over perovskite catalyst: A simulation study using experimental kinetic model
Yaghobi, Nakisa
Ghoreishy, Mir Hamid Reza
JOURNAL OF NATURAL GAS CHEMISTRY, 2008, 17 (01): : 8 - 16
[8] OXIDATIVE COUPLING OF METHANE IN A CIRCULAR FIXED BED REACTOR WITH 30 mL MgO/BaCO CATALYST
丁彦，丁雪加，王晓来，达建文，沈师孔
不详
Journal of Natural Gas Chemistry , 1998, (02)
[9] Oxidative coupling of methane in a fluidized-bed reactor over a highly active and selective catalyst
Mleczko, L
Pannek, U
Niemi, VM
Hiltunen, J
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1996, 35 (01) : 54 - 61
[10] CATALYST POISONING AND FIXED-BED REACTOR DYNAMICS
WENG, HS
EIGENBERGER, G
BUTT, JB
CHEMICAL ENGINEERING SCIENCE, 1975, 30 (11) : 1341 - 1351

← 1 2 3 4 5 →