BREAKDOWN OF GLOBAL COUPLING IN OSCILLATORY CHEMICAL-REACTIONS

被引:68
作者
MERTENS, F
IMBIHL, R
MIKHAILOV, A
机构
[1] Fritz Haber Institut der Max Planck Gesellschaft, 14195 Berlin (Dahlem), Faradayweg 4-6, D
关键词
D O I
10.1063/1.465590
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The effects of global coupling through the gas phase in oscillatory surface chemical reactions are investigated using a model which represents the complex Ginzburg-Landau equation with an additional integral term. Depending on the parameters of the model, global coupling is found to have either a synchronizing or desynchronizing effect. Respectively, the breakdown of global coupling requires the presence of strong supercritical inhomogeneities or spontaneously occurs in a uniform system.
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页码:8668 / 8671
页数:4
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