FEMTOSECOND PROCESSES AND ULTRAFAST BIOLOGICAL ELECTRON-TRANSFER

被引：3
|
作者：
SUZUKI, S
SUNG, HC
HAYASHI, M
LIN, SH
机构：
[1] ARIZONA STATE UNIV,DEPT CHEM & BIOCHEM,TEMPE,AZ 85287
[2] ARIZONA STATE UNIV,CTR EARLY EVENTS PHOTOSYNTH,TEMPE,AZ 85287
来源：
PHYSICA A | 1995年 / 221卷 / 1-3期
基金：
美国国家科学基金会;
关键词：
D O I：
10.1016/0378-4371(95)00226-W
中图分类号：
O4 [物理学];
学科分类号：
0702 ;
摘要：
In this paper, we report the calculated femtosecond transient spectra of the primary electron transfer in the bacterial reaction center of Rhodobacter sphaeroides R26. The excitation dependence of the time-resolved spectra is simulated. The effects of vibrational coherence on the time-resolved spectra are discussed. The electron transfer accompanying vibrational relaxation is theoretically investigated using the single-vibronic level electron transfer rate constants. The effects of multi-modes and temperature on the electron transfer rate constants are also reported.
引用
收藏
页码：15 / 29
页数：15
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