INCOMPLETE MELTING OF PB(001) AND VICINAL SURFACES

被引:46
作者
VANPINXTEREN, HM
FRENKEN, JWM
机构
[1] FOM-Institute for Atomic and Molecular Physics, 1098 SJ Amsterdam
关键词
D O I
10.1016/0039-6028(92)90810-S
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Medium energy ion scattering experiments on a cylindrically shaped Pb crystal demonstrate that at temperatures above 500 K, a finite amount of disorder develops at the Pb(001) surface and at vicinal surfaces with 5-degrees and 10-degrees miscut angle. The number of disordered atoms on these surfaces saturates between 1 and 0.05 K below the bulk melting point. The maximum amount of disorder increases with miscut angle from 1.3 ML on Pb(001) to 1.9 and 3.5 ML on the 5-degrees and 10-degrees vicinal surfaces, respectively. The observed scattered ion yields cannot be ascribed to mere anomalously strong surface vibrations. We conclude that these surfaces develop liquid-like disorder which can be interpreted as incomplete melting due to layering effects. The measurements show no sign of a prewetting transition up to (T(m) - 0.05 K). Furthermore, we have no indication of a surface-melting induced faceting transition of the two vicinal surfaces.
引用
收藏
页码:383 / 394
页数:12
相关论文
共 38 条
[1]  
ALKEMADE PFA, IN PRESS
[2]  
[Anonymous], 1988, PHASE TRANSITIONS CR
[3]  
[Anonymous], 1977, STOPPING RANGES IONS
[4]  
BILALBEGOVIC G, 1991, SURF SCI, V258, pL676, DOI 10.1016/0039-6028(91)90888-Y
[5]   ORIENTATIONAL PHASE-SEPARATION FOR VICINAL SURFACES CLOSE TO THE NONMELTING PB(111) FACE [J].
BILALBEGOVIC, G ;
ERCOLESSI, F ;
TOSATTI, E .
EUROPHYSICS LETTERS, 1992, 17 (04) :333-337
[6]  
CaO Y., PREPRINT
[7]   ANOMALOUS THERMAL-EXPANSION OF NI(001) [J].
CAO, YJ ;
CONRAD, E .
PHYSICAL REVIEW LETTERS, 1990, 65 (22) :2808-2811
[8]  
CHANDAVARKAR S, UNPUB
[9]   HAMAKER CONSTANT CALCULATIONS AND SURFACE MELTING OF METALS [J].
CHEN, XJ ;
LEVI, AC ;
TOSATTI, E .
SURFACE SCIENCE, 1991, 251 :641-644
[10]   WETTING AND SURFACE MELTING - CAPILLARY FLUCTUATIONS VS LAYERWISE SHORT-RANGE ORDER [J].
CHERNOV, AA ;
MIKHEEV, LV .
PHYSICA A, 1989, 157 (02) :1042-1058