EXPERIMENTAL-DETERMINATION OF THE QUANTUM-MECHANICAL STATE OF A MOLECULAR VIBRATIONAL-MODE USING FLUORESCENCE TOMOGRAPHY

被引：303
作者：
DUNN, TJ
WALMSLEY, IA
MUKAMEL, S
机构：
[1] UNIV ROCHESTER,INST OPT,ROCHESTER,NY 14627
[2] UNIV ROCHESTER,DEPT CHEM,ROCHESTER,NY 14627
来源：
PHYSICAL REVIEW LETTERS | 1995年 / 74卷 / 06期
关键词：
D O I：
10.1103/PhysRevLett.74.884
中图分类号：
O4 [物理学];
学科分类号：
0702 ;
摘要：
We present a spectroscopic method for the complete characterization of the quantum state of the vibrational mode of a molecule in terms of a phase-space quasiprobability distribution. The distribution for a molecular vibrational mode excited by a short optical pulse is reconstructed from measurements of its time-dependent spectrum of fluorescence. © 1995 The American Physical Society.
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页码：884 / 887
页数：4
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