OBSERVATION OF THE DARK EXCITON IN CDSE QUANTUM DOTS

被引:736
作者
NIRMAL, M [1 ]
NORRIS, DJ [1 ]
KUNO, M [1 ]
BAWENDI, MG [1 ]
EFROS, AL [1 ]
ROSEN, M [1 ]
机构
[1] USN,RES LAB,BEAM THEORY SECT,WASHINGTON,DC 20375
关键词
D O I
10.1103/PhysRevLett.75.3728
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We use external magnetic fields to identify the band edge emitting state in CdSe quantum dots. The field dependence of emission decays and LO phonon spectra show the importance of exciton spin dynamics in the recombination mechanism. To interpret our results we calculate the band edge exciton structure, including the effects of the electron-hole exchange interaction and a nonspherical shape. The exchange term, negligible in the bulk, is strongly enhanced by quantum confinement and allows the observation of an optically passive ''dark'' excitonic state.
引用
收藏
页码:3728 / 3731
页数:4
相关论文
共 24 条
[1]  
[Anonymous], 1975, HAYAT
[2]   LUMINESCENCE PROPERTIES OF CDSE QUANTUM CRYSTALLITES - RESONANCE BETWEEN INTERIOR AND SURFACE LOCALIZED STATES [J].
BAWENDI, MG ;
CARROLL, PJ ;
WILSON, WL ;
BRUS, LE .
JOURNAL OF CHEMICAL PHYSICS, 1992, 96 (02) :946-954
[4]   IDENTIFICATION OF RADIATIVE TRANSITIONS IN HIGHLY POROUS SILICON [J].
CALCOTT, PDJ ;
NASH, KJ ;
CANHAM, LT ;
KANE, MJ ;
BRUMHEAD, D .
JOURNAL OF PHYSICS-CONDENSED MATTER, 1993, 5 (07) :L91-L98
[5]  
CHAMARRO M, 1995, JPN J APPL PHYS S, V34, P12
[6]   BAND-EDGE ABSORPTION AND LUMINESCENCE OF NONSPHERICAL NANOMETER-SIZE CRYSTALS [J].
EFROS, AL ;
RODINA, AV .
PHYSICAL REVIEW B, 1993, 47 (15) :10005-10007
[7]   LUMINESCENCE POLARIZATION OF CDSE MICROCRYSTALS [J].
EFROS, AL .
PHYSICAL REVIEW B, 1992, 46 (12) :7448-7458
[8]  
EFROS AL, 1982, SOV PHYS SEMICOND+, V16, P772
[9]   ABSORPTION AND INTENSITY-DEPENDENT PHOTOLUMINESCENCE MEASUREMENTS ON CDSE QUANTUM DOTS - ASSIGNMENT OF THE 1ST ELECTRONIC-TRANSITIONS [J].
EKIMOV, AI ;
HACHE, F ;
SCHANNEKLEIN, MC ;
RICARD, D ;
FLYTZANIS, C ;
KUDRYAVTSEV, IA ;
YAZEVA, TV ;
RODINA, AV ;
EFROS, AL .
JOURNAL OF THE OPTICAL SOCIETY OF AMERICA B-OPTICAL PHYSICS, 1993, 10 (01) :100-107
[10]   DETECTION OF SHALLOW ELECTRON TRAPS IN QUANTUM SIZED CDS BY FLUORESCENCE QUENCHING EXPERIMENTS [J].
HASSELBARTH, A ;
EYCHMULLER, A ;
WELLER, H .
CHEMICAL PHYSICS LETTERS, 1993, 203 (2-3) :271-276