Preparation and characterization of graphene - TiO2 nanocomposite for enhanced photodegradation of Rhodamine-B dye

被引:61
作者
Ali, Mohamed H. H. [1 ]
Al-Afify, Afify D. [1 ]
Goher, Mohamed E. [1 ]
机构
[1] NIOF, Alexandria, Egypt
关键词
Photocatalysis; TiO2; Graphene oxide; Nanocomposite; XRD; Rh-B dye; TEM;
D O I
10.1016/j.ejar.2018.11.009
中图分类号
Q17 [水生生物学];
学科分类号
071004 ;
摘要
The synthesizing of TiO2@rGO nanocomposites using an efficient method has been carried out to enhance the photodegradation activities of TiO2. Reduced graphene oxide (rGO) synthesis has been illustrated as a key step. The preparation of TiO2@rGO is highly needed and recommended to develop an effective way for the reduction of GO. Our study illustrated an environmentally simple method for TiO2@rGO preparation and demonstrated its efficiency for photocatalytic process by utilizing rhodamine-B dye as an organic pollutant. Synthesized nanoparticles of reduced TiO2@rGO have an observable increase in photo-energy adsorption leading to the increase of the photodegradation reactions. From the obtained results, TiO2@rGO nanocomposites showed great ability to absorb photo-energy and enhance the photodegradation reactions. Moreover, the results revealed that the 3% TiO2@rGO have the best performance than 1% TiO2@rGO at pH = 9.0, 30 mg/l initial dye concentration and 60 min irradiation duration. The reduced graphene oxide production was considered as an influential co-catalyst for improving the TiO2 photocatalytic activities mainly owing to; the fast separation of h(+)/e and the adsorption improvement. Our study affirms the production of promising applicable particles using the environmental photocatalysis process in particular with regard to wastewater purification. (C) 2018 Hosting by Elsevier B.V. on behalf of National Institute of Oceanography and Fisheries.
引用
收藏
页码:263 / 270
页数:8
相关论文
共 50 条
  • [21] A ternary TiO2/WO3/graphene nanocomposite adsorbent: facile preparation and efficient removal of Rhodamine B
    Zhang, Yong-qiang
    Li, Xiao-hui
    Lu, Jie
    Si, Chong-dian
    Liu, Guang-jun
    Gao, Hong-tao
    Wang, Pi-bo
    INTERNATIONAL JOURNAL OF MINERALS METALLURGY AND MATERIALS, 2014, 21 (08) : 813 - 819
  • [22] PHOTOCATALYTIC DEGRADATION OF DYE OVER GRAPHENE-TiO2 NANOCOMPOSITE
    Nossol, Arlene B. S.
    Rosa, Suzamar M. C.
    Nossol, Edson
    Zarbin, Aldo J. G.
    Peralta-Zamora, Patricio
    QUIMICA NOVA, 2016, 39 (06): : 686 - 690
  • [23] Hierarchically assembled porous TiO2 nanoparticles with enhanced photocatalytic activity towards Rhodamine-B degradation
    Hiremath, Vishwanath
    Deonikar, Virendrakumar G.
    Kim, Hem
    Seo, Jeong Gil
    COLLOIDS AND SURFACES A-PHYSICOCHEMICAL AND ENGINEERING ASPECTS, 2020, 586
  • [24] Preparation, Characterization and Photocatalytic Activities of TiO2-coated Activated Carbon Catalysts for Rhodamine B Photodegradation
    Asilturk, Meltem
    Sener, Sadiye
    Sener, Engin
    BULLETIN OF THE KOREAN CHEMICAL SOCIETY, 2015, 36 (02): : 455 - 463
  • [25] Metal organic framework-derived C-doped ZnO/TiO2 nanocomposite catalysts for enhanced photodegradation of Rhodamine B
    Wang, Yingming
    Liu, Xiaoxiao
    Guo, Lin
    Shang, Linqing
    Ge, Shengsong
    Song, Gang
    Naik, Nithesh
    Shao, Qian
    Lin, Jing
    Guo, Zhanhu
    JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2021, 599 : 566 - 576
  • [26] Enhancement of visible light organic dyes photodegradation using TiO2 (001)/Graphene oxide nanocomposite
    Izzataddini, Arini
    Romdoni, Yoga
    Helmiyati
    Marantika, Rika Novi
    Amir, Zulhemi
    Kadja, Grandprix T. M.
    Jiwanti, Prastika K.
    Khalil, Munawar
    Jan, Badrul Mohamed
    INORGANIC CHEMISTRY COMMUNICATIONS, 2023, 157
  • [27] Construction of direct Z-scheme AgIO4/TiO2 heterojunctions for exceptional photodegradation of rhodamine B dye
    Ahmed, Mohamed A.
    Mahran, Blal Mohamed
    Abbas, Ahmed Mohamed
    Tarek, Mohamed Ahmed
    Saed, Ahmed Mohamed
    JOURNAL OF DISPERSION SCIENCE AND TECHNOLOGY, 2022, 43 (03) : 349 - 363
  • [28] Solar photodegradation of Rhodamine B dye by Cu2O/TiO2 heterostructure: experimental and computational studies of degradation and toxicity
    Messaadia, L.
    Kiamouche, S.
    Lahmar, H.
    Masmoudi, R.
    Boulahbel, H.
    Trari, M.
    Benamira, M.
    JOURNAL OF MOLECULAR MODELING, 2023, 29 (02)
  • [29] Preparation and characterization of a photocatalytic antibacterial material: Graphene oxide/TiO2/bacterial cellulose nanocomposite
    Liu, Ling-Pu
    Yang, Xiao-Ning
    Ye, Li
    Xue, Dong-Dong
    Liu, Miao
    Jia, Shi-Ru
    Hou, Ying
    Chu, Li-Qiang
    Zhong, Cheng
    CARBOHYDRATE POLYMERS, 2017, 174 : 1078 - 1086
  • [30] Photodegradation of rhodamine B under visible light by bimetal codoped TiO2 nanocrystals
    Wang, Zhuyi
    Chen, Cheng
    Wu, Fengqing
    Zou, Bo
    Zhao, Meng
    Wang, Jinxing
    Feng, Caihui
    JOURNAL OF HAZARDOUS MATERIALS, 2009, 164 (2-3) : 615 - 620