COLLECTIVE OPTICAL-RESPONSE OF MOLECULAR AGGREGATES

被引：40

作者：

FIDDER, H ^{[1
]}

WIERSMA, DA ^{[1
]}

机构：

[1] UNIV GRONINGEN,CTR MAT SCI,DEPT CHEM PHYS,ULTRAFAST LASER & SPECT LAB,9747 AG GRONINGEN,NETHERLANDS

来源：

PHYSICA STATUS SOLIDI B-BASIC RESEARCH | 1995年 / 188卷 / 01期

关键词：

D O I：

10.1002/pssb.2221880126

中图分类号：

O469 [凝聚态物理学];

学科分类号：

070205 ;

摘要：

Relative fluorescence quantum yield, fluorescence lifetime, optical dephasing, and absorption line shift data are presented for both excitonic transitions of the pseudoisocyanine (PIC) J-aggregate. The data indicate activation of the optical dephasing by exciton-acoustic phonon scattering at low temperatures. Above approximately 80 K the optical dephasing, line shift as well as the fluorescence lifetime lengthening call for activation by high frequency phonons. Moreover, resonance Raman data indicate the delocalization of low frequency vibrational modes in the aggregate.

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页码：285 / 295

页数：11

相关论文

共 34 条

[1] ONE-DIMENSIONAL VIBRATIONAL EXCITONS IN 1,2,4,5-TETRACHLOROBENZENE [J].

ABRAMSON, EH ;

JONGENELIS, APJM ;

SCHMIDT, J .

JOURNAL OF CHEMICAL PHYSICS, 1987, 87 (07) :3719-3723

[2] INHOMOGENEOUS BROADENING IN EXCITONIC SYSTEMS [J].

BOUKAHIL, A ;

HUBER, DL .

JOURNAL OF LUMINESCENCE, 1990, 45 (1-6) :13-16

[3] SINGLET EXCITON ANNIHILATION IN THE PICOSECOND FLUORESCENCE DECAY OF 1,1'-DIETHYL-2,2'-CYANINE CHLORIDE DYE J-AGGREGATE [J].

BRUMBAUGH, DV ;

MUENTER, AA ;

KNOX, W ;

MOUROU, G ;

WITTMERSHAUS, B .

JOURNAL OF LUMINESCENCE, 1984, 31-2 (DEC) :783-785

[4] Multiplet structure of aggregated states in 1,1 '-diethyl-2,2 '-cyanine dye [J].

Cooper, W. .

CHEMICAL PHYSICS LETTERS, 1970, 7 (01) :73-77

[5] DISPERSION AND RESONANCE TERMS IN EXCITON-PHONON COUPLING - ABSORPTION-BAND PROFILES IN MOLECULAR-CRYSTALS [J].

CRAIG, DP ;

DISSADO, LA .

CHEMICAL PHYSICS, 1976, 14 (01) :89-110

[6]

Davydov A. S., 1971, THEORY MOL EXCITONS

[7] OPTICAL-DYNAMICS OF CONDENSED MOLECULAR AGGREGATES - AN ACCUMULATED PHOTON-ECHO AND HOLE-BURNING STUDY OF THE J-AGGREGATE [J].

DEBOER, S ;

VINK, KJ ;

WIERSMA, DA .

CHEMICAL PHYSICS LETTERS, 1987, 137 (02) :99-106

[8] DEPHASING-INDUCED DAMPING OF SUPERRADIANT EMISSION IN J-AGGREGATES [J].

DEBOER, S ;

WIERSMA, DA .

CHEMICAL PHYSICS LETTERS, 1990, 165 (01) :45-53

[9] LINEWIDTH DEPENDENCE OF RADIATIVE EXCITON LIFETIMES IN QUANTUM-WELLS [J].

FELDMANN, J ;

PETER, G ;

GOBEL, EO ;

DAWSON, P ;

MOORE, K ;

FOXON, C ;

ELLIOTT, RJ .

PHYSICAL REVIEW LETTERS, 1987, 59 (20) :2337-2340

[10] RESONANCE-LIGHT-SCATTERING STUDY AND LINE-SHAPE SIMULATION OF THE J-BAND [J].

FIDDER, H ;

WIERSMA, DA .

PHYSICAL REVIEW LETTERS, 1991, 66 (11) :1501-1504

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