MUTUALLY COUPLED OSCILLATORS WITH TIME-DELAY

被引:41
|
作者
WEINER, J
HOLZ, R
SCHNEIDER, FW
BARELI, K
机构
[1] UNIV WURZBURG,INST PHYS CHEM,MARCUSSTR 9-11,W-8700 WURZBURG,GERMANY
[2] TEL AVIV UNIV,SACKLER FAC EXACT SCI,SCH CHEM,IL-69978 TEL AVIV,ISRAEL
来源
JOURNAL OF PHYSICAL CHEMISTRY | 1992年 / 96卷 / 22期
关键词
D O I
10.1021/j100201a041
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We present a system of two identical chemical oscillators which are coupled by means of their flow rates. The individual flow rate of one oscillator is controlled by the output of the other oscillator and vice versa. A delay time is applied between the output of one oscillator and the input to the other one. This delay has been investigated both theoretically and experimentally for the minimal bromate oscillator. By variation of the delay time both oscillators dramatically change their periods and amplitudes. At lower coupling strengths, the periods of both oscillators increase and decrease in a sawtooth fashion with increasing delay times. At high coupling strengths multimode patterns were obtained at high delay times. No quasiperiodic or aperiodic behavior was observed in this coupled system. The experimental results are in general agreement with those calculated with the Noyes-Field-Thompson mechanism.
引用
收藏
页码:8915 / 8919
页数:5
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