CLUSTER MATTER - THE TRANSITION OF OPTICAL ELASTIC-SCATTERING TO REGULAR REFLECTION

被引:48
作者
DUSEMUND, B [1 ]
HOFFMANN, A [1 ]
SALZMANN, T [1 ]
KREIBIG, U [1 ]
SCHMID, G [1 ]
机构
[1] UNIV ESSEN GESAMTHSCH,W-4300 ESSEN 1,GERMANY
来源
ZEITSCHRIFT FUR PHYSIK D-ATOMS MOLECULES AND CLUSTERS | 1991年 / 20卷 / 1-4期
关键词
D O I
10.1007/BF01543997
中图分类号
O64 [物理化学(理论化学)、化学物理学]; O56 [分子物理学、原子物理学];
学科分类号
070203 ; 070304 ; 081704 ; 1406 ;
摘要
The optical response of many-cluster systems (cluster matter) depends strongly on the mean filling factor and on its local variations. This is shown from Au clusters of various sizes which form coagulation systems. Measured spectra of the extinction, the absorbance, the integral scattering, the angle resolved scattering, the regular reflection and corresponding TEM micrographs are presented. It is demonstrated that by varying f from 10(-6) to 0.5 the incoherent Mie scattering is transformed into regular geometric-optical transmission and reflection ("Oseen-transition") while the spectral features even of the most densely packed samples still differ strongly from those of a bulk Au film.
引用
收藏
页码:305 / 308
页数:4
相关论文
共 4 条
  • [1] BORN M, 1985, OPTIK
  • [2] MANY-PARTICLE SYSTEMS - MODELS OF INHOMOGENEOUS MATTER
    KREIBIG, U
    QUINTEN, M
    SCHOENAUER, D
    [J]. PHYSICA A, 1989, 157 (01): : 244 - 261
  • [3] MANY-CLUSTER-SYSTEMS - MODELS OF INHOMOGENEOUS MATTER
    KREIBIG, U
    FAUTH, K
    QUINTEN, M
    SCHONAUER, D
    [J]. ZEITSCHRIFT FUR PHYSIK D-ATOMS MOLECULES AND CLUSTERS, 1989, 12 (1-4): : 505 - 514
  • [4] ELECTRONIC EXCITATIONS IN MANY-PARTICLE SYSTEMS - A QUANTITATIVE-ANALYSIS
    QUINTEN, M
    SCHONAUER, D
    KREIBIG, U
    [J]. ZEITSCHRIFT FUR PHYSIK D-ATOMS MOLECULES AND CLUSTERS, 1989, 12 (1-4): : 521 - 525