ANALYSIS OF THE LUMPED AND DISTRIBUTED OPTIMAL TEMPERATURE TRAJECTORIES FOR PACKED-BED REACTORS WITH CONCENTRATION DEPENDENT CATALYST DEACTIVATION

被引:5
作者
GONZALEZVELASCO, JR
GUTIERREZORTIZ, MA
GUTIERREZORTIZ, JI
GONZALEZMARCOS, JA
机构
[1] Departamento de Ingeniería Química, Facultad de Ciencias, Universidad del País Vasco, Bibao, E-48080
关键词
catalyst deactivation; control; distributed control; optimal control; temperature control;
D O I
10.1002/cjce.5450680517
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Algorithms published previously by the authors for solving the problem of spatially uniform and non‐uniform temperature optimal control in tubular fixed bed reactors have been applied to three systems with series catalyst deactivation and different ratios between the activation energies of the main and deactivation reactions. The optimal temperature and conversion trajectories as well as the maximum production obtained have been compared at the same final duration of operation. Systems with slow deactivation obtain maximum production with spatially uniform control, whilst for systems with rapid deactivation the temperature trajectory distributed both in space and time improves the production obtained with lumped control. Copyright © 1990 Canadian Society for Chemical Engineering
引用
收藏
页码:860 / 866
页数:7
相关论文
共 34 条
[1]   CONTROL OPTIMIZATION OF TUBULAR CATALYTIC REACTORS WITH CATALYST DECAY [J].
BUZZIFERRARIS, G ;
FACCHI, E ;
FORZATTI, P ;
TRONCONI, E .
INDUSTRIAL & ENGINEERING CHEMISTRY PROCESS DESIGN AND DEVELOPMENT, 1984, 23 (01) :126-131
[2]   OPTIMUM TEMPERATURE POLICY FOR A DEACTIVATING CATALYTIC PACKED-BED REACTOR [J].
CROWE, CM .
CHEMICAL ENGINEERING SCIENCE, 1979, 34 (09) :1176-1176
[3]   OPTIMIZATION OF REACTORS WITH CATALYST DECAY AND CONSTANT CONVERSION POLICY [J].
CROWE, CM .
CHEMICAL ENGINEERING SCIENCE, 1976, 31 (10) :959-962
[4]   OPTIMIZATION OF REACTORS WITH CATALYST DECAY .3. TUBULAR REACTOR WITH SEVERAL BEDS OF UNIFORM TEMPERATURE [J].
CROWE, CM ;
LEE, SI .
CANADIAN JOURNAL OF CHEMICAL ENGINEERING, 1971, 49 (03) :385-&
[6]   OPTIMIZATION BY DISTRIBUTED CONTROL OF REACTORS WITH DECAYING CATALYST .2. FIRST-ORDER CATALYST DEACTIVATION [J].
CROWE, CM ;
THERIEN, N .
CANADIAN JOURNAL OF CHEMICAL ENGINEERING, 1974, 52 (06) :822-829
[7]   OPTIMIZATION OF AN NORMAL-PENTANE ISOMERIZATION REACTOR [J].
CULFAZ, M ;
AKYURTLU, J ;
AKTAS, Z .
CHEMICAL ENGINEERING JOURNAL AND THE BIOCHEMICAL ENGINEERING JOURNAL, 1984, 28 (01) :39-48
[8]   DEHYDROGENATION OF 1-BUTENE INTO BUTADIENE - KINETICS, CATALYST COKING, AND REACTOR DESIGN [J].
DUMEZ, FJ ;
FROMENT, GF .
INDUSTRIAL & ENGINEERING CHEMISTRY PROCESS DESIGN AND DEVELOPMENT, 1976, 15 (02) :291-301
[9]   SPACE-TIME POLICY IN DEACTIVATING ISOTHERMAL CATALYST BEDS [J].
GONZALEZVALASCO, JR ;
GUTIERREZORTIZ, MA ;
GUTIERREZORTIZ, JI ;
ROMERO, A .
CHEMICAL ENGINEERING SCIENCE, 1984, 39 (03) :615-618
[10]   THE CONTROL OF THE TEMPERATURE AND THE FEED IN DEACTIVATING ISOTHERMAL CATALYST BEDS [J].
GONZALEZVELASCO, JR ;
GUTIERREZORTIZ, MA ;
GUTIERREZORTIZ, JI ;
ROMERO, A .
CHEMICAL ENGINEERING JOURNAL AND THE BIOCHEMICAL ENGINEERING JOURNAL, 1984, 28 (01) :13-20