PHASE-SEPARATION TO ANTIFERROMAGNETIC AND SUPERCONDUCTING DOMAINS IN OXYGEN-RICH SINGLE-CRYSTAL LA2CUO4+X - MAGNETIC AND STRUCTURAL NEUTRON-DIFFRACTION STUDIES

被引:35
作者
VAKNIN, D
ZARESTKY, JL
JOHNSTON, DC
SCHIRBER, JE
FISK, Z
机构
[1] IOWA STATE UNIV SCI & TECHNOL,AMES,IA 50011
[2] SANDIA NATL LABS,ALBUQUERQUE,NM 87185
[3] LOS ALAMOS NATL LAB,LOS ALAMOS,NM 87545
来源
PHYSICAL REVIEW B | 1994年 / 49卷 / 13期
关键词
D O I
10.1103/PhysRevB.49.9057
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We report on magnetic and structural neutron-diffraction studies of single-crystal La2CuO4+x versus temperature. The low-temperature diffraction data are consistent with the coexistence of two structurally related phases: nearly stoichiometric, antiferromagnetic (AF) domains, with average domain diameter approximately 500 angstrom in the CuO2 plane, and oxygen-rich, metallic, and superconducting domains. The ordered magnetic moment in the AF domains does not saturate at 10 K, and is on average, mu = (0.3 +/- 0.05)mu(B)/Cu atom. The phase-separation transition to these two phases occurs at T(PS) = 260 +/- 5 K, which is about 15 K higher than the Neel temperature, T(N) = 245 +/- 3 K. The value of T(PS) is identical within the errors with that (259 +/- 2 K) found previously from specific-heat. measurements on the same crystal. The structural properties of the single crystal are discussed and compared to those of polycrystalline oxygen-rich La2CuO4+x.
引用
收藏
页码:9057 / 9063
页数:7
相关论文
共 30 条
[1]   MAGNETIC PHASE-DIAGRAM AND MAGNETIC PAIRING IN DOPED LA2CUO4 [J].
AHARONY, A ;
BIRGENEAU, RJ ;
CONIGLIO, A ;
KASTNER, MA ;
STANLEY, HE .
PHYSICAL REVIEW LETTERS, 1988, 60 (13) :1330-1333
[2]   MAGNETIC-PROPERTIES OF THE SUPERCONDUCTING SUPEROXIDE LA2CUO4+DELTA [J].
ANSALDO, EJ ;
BREWER, JH ;
RISEMAN, TM ;
SCHIRBER, JE ;
VENTURINI, EL ;
MOROSIN, B ;
GINLEY, DS ;
STERNLIEB, B .
PHYSICAL REVIEW B, 1989, 40 (04) :2555-2557
[3]  
BEDNORZ JG, 1986, Z PHYS B, V64, P89
[4]   BULK SUPERCONDUCTIVITY AT 36 K IN LA1.8SR0.2CUO4 [J].
CAVA, RJ ;
VANDOVER, RB ;
BATLOGG, B ;
RIETMAN, EA .
PHYSICAL REVIEW LETTERS, 1987, 58 (04) :408-410
[5]   THE CRYSTAL-STRUCTURE OF SUPERCONDUCTING LA2CUO4.032 BY NEUTRON-DIFFRACTION [J].
CHAILLOUT, C ;
CHEONG, SW ;
FISK, Z ;
LEHMANN, MS ;
MAREZIO, M ;
MOROSIN, B ;
SCHIRBER, JE .
PHYSICA C, 1989, 158 (1-2) :183-191
[6]   2-PHASE STRUCTURAL REFINEMENT OF LA2CUO4.032 AT 15 K [J].
CHAILLOUT, C ;
CHENAVAS, J ;
CHEONG, SW ;
FISK, Z ;
MAREZIO, M ;
MOROSIN, B ;
SCHIRBER, JE .
PHYSICA C, 1990, 170 (1-2) :87-94
[7]   PHASE-SEPARATION AND FINITE SIZE SCALING IN LA2-XSRXCUO4+DELTA[0-LESS-THAN-OR-EQUAL-TO(X,DELTA)LESS-THAN-OR-EQUAL-TO-0.03] [J].
CHO, JH ;
CHOU, FC ;
JOHNSTON, DC .
PHYSICAL REVIEW LETTERS, 1993, 70 (02) :222-225
[8]   SPIN DYNAMICS IN LA2-XSRXCUO4 (0.02-LESS-THAN-OR-EQUAL-TO-X-LESS-THAN-OR-EQUAL-TO-0.08) FROM LA-139 NQR RELAXATION - FLUCTUATIONS IN A FINITE-LENGTH-SCALE SYSTEM [J].
CHO, JH ;
BORSA, F ;
JOHNSTON, DC ;
TORGESON, DR .
PHYSICAL REVIEW B, 1992, 46 (05) :3179-3182
[9]   MAGNETIC PHASE-DIAGRAM OF LIGHTLY DOPED LA2-XSRXCUO4 FROM LA-139 NUCLEAR-QUADRUPOLE RESONANCE [J].
CHOU, FC ;
BORSA, F ;
CHO, JH ;
JOHNSTON, DC ;
LASCIALFARI, A ;
TORGESON, DR ;
ZIOLO, J .
PHYSICAL REVIEW LETTERS, 1993, 71 (14) :2323-2326
[10]   FRUSTRATED ELECTRONIC PHASE-SEPARATION AND HIGH-TEMPERATURE SUPERCONDUCTORS [J].
EMERY, VJ ;
KIVELSON, SA .
PHYSICA C-SUPERCONDUCTIVITY AND ITS APPLICATIONS, 1993, 209 (04) :597-621