PHASE-CONTROL IN THE 2-COLOR PHOTODISSOCIATION OF HD+

被引：247
作者：
SHEEHY, B
WALKER, B
DIMAURO, LF
机构：
[1] Chemistry Department, Brookhaven National Laboratory, Upton
来源：
PHYSICAL REVIEW LETTERS | 1995年 / 74卷 / 24期
关键词：
D O I：
10.1103/PhysRevLett.74.4799
中图分类号：
O4 [物理学];
学科分类号：
0702 ;
摘要：
We report on the use of the relative phase between a two-color optical field (1053 and 527 nm) to coherently control the photodissociation of the HD+ molecule. The field-induced spatial asymmetry in the fragment spectrum shows a strong phase dependence, while no selectivity is produced in nearly isoenergetic channels. The positively charged fragments are observed to preferentially dissociate in a direction counterintuitive to classical expectations. © 1995 The American Physical Society.
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页码：4799 / 4802
页数：4
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