GROUND SPIN STATE VARIABILITY IN [FE4S4(SR)4]3- - SYNTHETIC ANALOGS OF THE REDUCED CLUSTERS IN FERREDOXINS AND OTHER IRON SULFUR PROTEINS - CASES OF EXTREME SENSITIVITY OF ELECTRONIC STATE AND STRUCTURE TO EXTRINSIC FACTORS

被引:148
作者
CARNEY, MJ
PAPAEFTHYMIOU, GC
SPARTALIAN, K
FRANKEL, RB
HOLM, RH
机构
[1] HARVARD UNIV, DEPT CHEM, CAMBRIDGE, MA 02138 USA
[2] MIT, FRANCIS BITTER NATL MAGNET LAB, CAMBRIDGE, MA 02139 USA
关键词
D O I
10.1021/ja00226a025
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
引用
收藏
页码:6084 / 6095
页数:12
相关论文
共 67 条
[1]   ANALYSIS OF THE HIGH-SPIN STATES OF THE 2[4FE-4SE]+ FERREDOXIN FROM CLOSTRIDIUM-PASTEURIANUM BY MOSSBAUER-SPECTROSCOPY [J].
AURIC, P ;
GAILLARD, J ;
MEYER, J ;
MOULIS, JM .
BIOCHEMICAL JOURNAL, 1987, 242 (02) :525-530
[2]   THEORETICAL STUDIES OF GROUND AND EXCITED-STATES OF A MODEL OF ACTIVE-SITE IN OXIDIZED AND REDUCED RUBREDOXIN [J].
BAIR, RA ;
GODDARD, WA .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1978, 100 (18) :5669-5676
[3]  
Berg J.M., 1982, METAL IONS BIOL, V4
[4]   CRYSTAL-STRUCTURE OF [(C2H5)4N]3[FE4S4(SCH2PH)4], A REDUCED FERREDOXIN SITE ANALOG WITH A NONTETRAGONAL FE4S4 CORE STRUCTURE IN THE SOLID-STATE [J].
BERG, JM ;
HODGSON, KO ;
HOLM, RH .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1979, 101 (16) :4586-4593
[5]   ELECTRON SPIN-LATTICE RELAXATION OF THE (4FE-4S) FERREDOXIN FROM B-STEAROTHERMOPHILUS - COMPARISON WITH OTHER IRON PROTEINS [J].
BERTRAND, P ;
GAYDA, JP ;
RAO, KK .
JOURNAL OF CHEMICAL PHYSICS, 1982, 76 (10) :4715-4719
[6]   INORGANIC DERIVATIVES OF IRON-SULFIDE-THIOLATE DIMERS AND TETRAMERS - STRUCTURES OF TETRACHLORO-MU-DISULFIDO-DIFERRATE(III) AND TETRAKIS(CHLORO-MU-3-SULFIDO-IRON) DIANIONS [J].
BOBRIK, MA ;
HODGSON, KO ;
HOLM, RH .
INORGANIC CHEMISTRY, 1977, 16 (08) :1851-1858
[7]  
CAMBRAY J, 1977, INORG CHEM, V16, P2656
[8]   DEMONSTRATION OF ALTERNATIVE SPIN STATES IN CLUSTERS CONTAINING THE BIOLOGICALLY RELEVANT [FE4S4]1+ CORE [J].
CARNEY, MJ ;
HOLM, RH ;
PAPAEFTHYMIOU, GC ;
FRANKEL, RB .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1986, 108 (12) :3519-3521
[9]   ALTERNATIVE SPIN STATES IN SYNTHETIC ANALOGS OF BIOLOGICAL CLUSTERS - SPIN-QUARTET GROUND-STATES AND STRUCTURES OF [FE4S4(SPH)4]3- AND [FE4SE4(SPH)4]3- AS THEIR TETRAMETHYLAMMONIUM SALTS [J].
CARNEY, MJ ;
PAPAEFTHYMIOU, GC ;
WHITENER, MA ;
SPARTALIAN, K ;
FRANKEL, RB ;
HOLM, RH .
INORGANIC CHEMISTRY, 1988, 27 (02) :346-352
[10]  
CARNEY MJ, 1988, THESIS HARVARD U