TRANSITION BETWEEN FRONTS AND SPIRAL WAVES IN A BISTABLE SURFACE-REACTION

被引:54
作者
BAR, M
NETTESHEIM, S
ROTERMUND, HH
EISWIRTH, M
ERTL, G
机构
[1] Fritz-Haber-Institut der Max-Planck-Gesellschaft, D-14195 Berlin
关键词
D O I
10.1103/PhysRevLett.74.1246
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The transition between wave fronts and spiral waves in the CO oxidation on a Pt(110) surface has been investigated by means of photoemission electron microscopy and treated theoretically by simulations with a reaction-diffusion model under bistable conditions. Periodic external forcing of spirals near the transition to front behavior led to a complex pattern best characterized as a pulsating spiral-front hybrid, thus confirming the bistable nature of the underlying reaction kinetics. © 1995 The American Physical Society.
引用
收藏
页码:1246 / 1249
页数:4
相关论文
共 21 条
[1]   SPIRAL WAVES IN A SURFACE-REACTION - MODEL-CALCULATIONS [J].
BAR, M ;
GOTTSCHALK, N ;
EISWIRTH, M ;
ERTL, G .
JOURNAL OF CHEMICAL PHYSICS, 1994, 100 (02) :1202-1214
[2]   EXPERIMENTAL-EVIDENCE OF A SUSTAINED STANDING TURING-TYPE NONEQUILIBRIUM CHEMICAL-PATTERN [J].
CASTETS, V ;
DULOS, E ;
BOISSONADE, J ;
DEKEPPER, P .
PHYSICAL REVIEW LETTERS, 1990, 64 (24) :2953-2956
[3]   PATTERN-FORMATION OUTSIDE OF EQUILIBRIUM [J].
CROSS, MC ;
HOHENBERG, PC .
REVIEWS OF MODERN PHYSICS, 1993, 65 (03) :851-1112
[4]   A UHV-COMPATIBLE PHOTOELECTRON EMISSION MICROSCOPE FOR APPLICATIONS IN SURFACE SCIENCE [J].
ENGEL, W ;
KORDESCH, ME ;
ROTERMUND, HH ;
KUBALA, S ;
VONOERTZEN, A .
ULTRAMICROSCOPY, 1991, 36 (1-3) :148-153
[5]   OSCILLATORY KINETICS AND SPATIOTEMPORAL SELF-ORGANIZATION IN REACTIONS AT SOLID-SURFACES [J].
ERTL, G .
SCIENCE, 1991, 254 (5039) :1750-1755
[6]   EFFECTS OF BOUNDARIES ON PATTERN-FORMATION - CATALYTIC-OXIDATION OF CO ON PLATINUM [J].
GRAHAM, MD ;
KEVREKIDIS, IG ;
ASAKURA, K ;
LAUTERBACH, J ;
KRISCHER, K ;
ROTERMUND, HH ;
ERTL, G .
SCIENCE, 1994, 264 (5155) :80-82
[7]   DOMAIN-WALLS IN NONEQUILIBRIUM SYSTEMS AND THE EMERGENCE OF PERSISTENT PATTERNS [J].
HAGBERG, A ;
MERON, E .
PHYSICAL REVIEW E, 1993, 48 (02) :705-708
[8]   FROM LABYRINTHINE PATTERNS TO SPIRAL TURBULENCE [J].
HAGBERG, A ;
MERON, E .
PHYSICAL REVIEW LETTERS, 1994, 72 (15) :2494-2497
[9]   STABLY PROPAGATING PERIODIC-WAVES IN INTRINSICALLY BISTABLE REACTION-DIFFUSION SYSTEMS [J].
KOGA, S .
PROGRESS OF THEORETICAL PHYSICS, 1993, 90 (06) :1361-1366
[10]   OSCILLATORY CO OXIDATION ON PT(110) - MODELING OF TEMPORAL SELF-ORGANIZATION [J].
KRISCHER, K ;
EISWIRTH, M ;
ERTL, G .
JOURNAL OF CHEMICAL PHYSICS, 1992, 96 (12) :9161-9172