ANOMALIES IN THE SCALING OF THE DIELECTRIC ALPHA-RELAXATION

被引:208
作者
SCHONHALS, A [1 ]
KREMER, F [1 ]
HOFMANN, A [1 ]
FISCHER, EW [1 ]
SCHLOSSER, E [1 ]
机构
[1] MAX PLANCK INST POLYMER RES, W-6500 MAINZ, GERMANY
关键词
D O I
10.1103/PhysRevLett.70.3459
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
By measuring the complex dielectric function over 15 decades in frequency we evaluate the scaling of the alpha-relaxation for several glass-forming liquids including propylene carbonate. The temperature dependence of the mean relaxation time and of the relaxation strength of the relaxation function displays two dynamical regions being separated by a crossover temperature. The observed findings are essentially not in accordance with predictions of the mode-coupling theory and light scattering results for propylene carbonate [M. Elmroth et al., Phys. Rev. Lett. 68, 79 (1992)].
引用
收藏
页码:3459 / 3462
页数:4
相关论文
共 31 条
[1]   ON TEMPERATURE DEPENDENCE OF COOPERATIVE RELAXATION PROPERTIES IN GLASS-FORMING LIQUIDS [J].
ADAM, G ;
GIBBS, JH .
JOURNAL OF CHEMICAL PHYSICS, 1965, 43 (01) :139-&
[2]  
BENTZELIUS U, 1984, J PHYS C SOLID STATE, V17, P5915
[3]   NEUTRON AND LIGHT-SCATTERING STUDY OF RELAXATION DYNAMICS IN A GLASS-FORMING FRAGILE MOLECULAR LIQUID [J].
BORJESSON, L ;
ELMROTH, M ;
TORELL, LM .
CHEMICAL PHYSICS, 1990, 149 (1-2) :209-220
[4]   FLUCTUATING NONLINEAR HYDRODYNAMICS AND THE LIQUID-GLASS TRANSITION [J].
DAS, SP ;
MAZENKO, GF .
PHYSICAL REVIEW A, 1986, 34 (03) :2265-2282
[5]   STRUCTURAL RELAXATION BY DIGITAL-CORRELATION SPECTROSCOPY [J].
DEMOULIN, C ;
MONTROSE, CJ ;
OSTROWSKY, N .
PHYSICAL REVIEW A, 1974, 9 (04) :1740-1742
[6]   SPECIFIC-HEAT SPECTROSCOPY AND DIELECTRIC SUSCEPTIBILITY MEASUREMENTS OF SALOL AT THE GLASS-TRANSITION [J].
DIXON, PK .
PHYSICAL REVIEW B, 1990, 42 (13) :8179-8186
[7]   CHARACTERISTIC LENGTH OF GLASS-TRANSITION [J].
DONTH, E .
JOURNAL OF NON-CRYSTALLINE SOLIDS, 1991, 131 :204-206
[8]  
DONTH E, 1981, GLASUIUMLBERGANG
[9]   OBSERVATION OF A DYNAMIC ANOMALY IN THE LIQUID-GLASS TRANSFORMATION RANGE BY BRILLOUIN-SCATTERING [J].
ELMROTH, M ;
BORJESSON, L ;
TORELL, LM .
PHYSICAL REVIEW LETTERS, 1992, 68 (01) :79-82
[10]   TEMPERATURE-DEPENDENCE OF CHARACTERISTIC LENGTH FOR GLASS-TRANSITION [J].
FISCHER, EW ;
DONTH, E ;
STEFFEN, W .
PHYSICAL REVIEW LETTERS, 1992, 68 (15) :2344-2346