SINGLE-PARTICLE AND COLLECTIVE DEGREES OF FREEDOM IN C-60

被引:64
作者
ALASIA, F
BROGLIA, RA
ROMAN, HE
SERRA, L
COLO, G
PACHECO, JM
机构
[1] UNIV MILAN,DIPARTIMENTO FIS,I-20133 MILAN,ITALY
[2] UNIV COPENHAGEN,NIELS BOHR INST,DK-2100 COPENHAGEN O,DENMARK
[3] UNIV GIESSEN,INST THEORET PHYS,D-35392 GIESSEN,GERMANY
[4] INST PHYS NUCL LYON,DIV PHYS THEOR,F-91406 ORSAY,FRANCE
[5] UNIV COIMBRA,DEPT FIS,P-3000 COIMBRA,PORTUGAL
关键词
D O I
10.1088/0953-4075/27/18/006
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
The electromagnetic response of the fullerene C-60 in the energy range 0 less than or equal to E less than or equal to 35 eV, exhausting 84% of the Thomas-Reiche-Kuhn sum rule, has been worked out using the local density and random phase approximations. A detailed correspondence between the calculated pi-plasmons and the peaks determined in optical/uv studies is found. The damping width (approximate to 12 eV) of the Mie resonance observed at approximate to 20 eV is well reproduced, and is due to Landau damping. This resonance is found to be determined by sigma --> sigma and, to a large extent, also by sigma --> pi, delta particle-hole transitions.
引用
收藏
页码:L643 / L649
页数:7
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