NONLINEAR OPTICAL-PROPERTIES OF H-2 AND D-2

被引：33
|
作者：
BISHOP, DM
PIPIN, J
RERAT, M
机构：
[1] Department of Chemistry, University of Ottawa, Ottawa
[2] Equipe de Recherche (474) Associée au CNRS, Université de Pau
来源：
JOURNAL OF CHEMICAL PHYSICS | 1990年 / 92卷 / 03期
关键词：
D O I：
10.1063/1.458072
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Accurate wave functions of the James-Coolidge type, which account for electron correlation, are used to calculate for H2 and D2 the dynamic second hyperpolarizabilities (γ) which mediate the nonlinear optical processes: dc Kerr, dc electric-field-induced second-harmonic generation and third-harmonic generation. Values are given for a range of frequencies (ω = 0 to ω = 0.05 a.u.) as well as for some common laser frequencies. The effects of vibration are explicitly considered. As well, values of the dynamic field-gradient polarizabilities B and C are found. The results are more accurate than those previously published. © 1990 American Institute of Physics.
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页码：1902 / 1908
页数：7
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