FORMALIZED QUANTUM-MECHANICAL FLOQUET THEORY AND ITS APPLICATION TO SAMPLE-SPINNING IN NUCLEAR-MAGNETIC-RESONANCE

被引：106
作者：
LEVANTE, TO
BALDUS, M
MEIER, BH
ERNST, RR
机构：
[1] Laboratorium für Physikalische Chemie, Eidgenössische Technische Hochschule, Zürich
[2] NSR Center for Molecular Structure, Design, and Synthesis, Laboratory of Physical Chemistry, University of Nijmegen, Nijmegen, NL-6525 ED, Toernooiveld
来源：
MOLECULAR PHYSICS | 1995年 / 86卷 / 05期
关键词：
D O I：
10.1080/00268979500102671
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Quantum mechanical Floquet theory, a powerful tool for the solution of Schrodinger equations with a periodically time-dependent Hamiltonian is formalized by the systematic usage of the Floquet Hilbert space, the Floquet density operator, Floquet detection operators, and of the Floquet Liouville space. A concise description is obtained that is useful in analytical calculations and for computer simulations. It is implemented in the context of the general computational environment 'GAMMA'. Simplified expressions are derived for single-axis and double-axis sample-spinning experiments in NMR.
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页码：1195 / 1212
页数：18
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