Single-walled carbon nanotubes as excitonic optical wires

被引:53
作者
Joh, Daniel Y. [1 ,2 ]
Kinder, Jesse [2 ]
Herman, Lihong H. [1 ]
Ju, Sang-Yong [2 ]
Segal, Michael A. [2 ]
Johnson, Jeffreys N. [2 ]
Chan, Garnet K. -L. [2 ]
Park, Jiwoong [2 ,3 ]
机构
[1] Cornell Univ, Sch Appl & Engn Phys, Ithaca, NY 14853 USA
[2] Cornell Univ, Dept Chem & Chem Biol, Ithaca, NY 14853 USA
[3] Cornell Univ, Kavli Inst Cornell Nanoscale Sci, Ithaca, NY 14853 USA
基金
美国国家科学基金会;
关键词
ANTENNAS; SPECTROSCOPY; SCATTERING; SPECTRA;
D O I
10.1038/NNANO.2010.248
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Although metallic nanostructures are useful for nanoscale optics, all of their key optical properties are determined by their geometry. This makes it difficult to adjust these properties independently, and can restrict applications. Here we use the absolute intensity of Rayleigh scattering to show that single-walled carbon nanotubes can form ideal optical wires. The spatial distribution of the radiation scattered by the nanotubes is determined by their shape, but the intensity and spectrum of the scattered radiation are determined by exciton dynamics, quantum-dot-like optical resonances and other intrinsic properties. Moreover, the nanotubes display a uniform peak optical conductivity of similar to 8 e(2)/h, which we derive using an exciton model, suggesting universal behaviour similar to that observed in nanotube conductance. We further demonstrate a radiative coupling between two distant nanotubes, with potential applications in metamaterials and optical antennas.
引用
收藏
页码:51 / 56
页数:6
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