Light-induced switching between singlet and triplet superconducting states

While the search for topological triplet-pairing superconductivity has remained a challenge, recent developments in optically stabilizing metastable superconducting states suggest a new route to realizing this elusive phase. Here, we devise a testable theory of competing superconducting orders that permits ultrafast switching to an opposite-parity superconducting phase in centrosymmetric crystals with strong spin-orbit coupling. Using both microscopic and phenomenological models, we show that dynamical inversion symmetry breaking with a tailored light pulse can induce odd-parity (spin triplet) order parameter oscillations in a conventional even-parity (spin singlet) superconductor, which when driven strongly can send the system to a competing minimum in its free energy landscape. Our results provide new guiding principles for engineering unconventional electronic phases using light, suggesting a fundamentally non-equilibrium route toward realizing topological superconductivity. S. Gassner et al. propose using light pulses to drive a centrosymmetric s-wave superconductor with strong spin-orbit coupling into a metastable triplet p-wave superconductor with non-trivial topology. The two superconducting orders must be closely competing in equilibrium and the light pulse must break a generalized, dynamic form of inversion symmetry.