Antiferromagnetic resonance and high magnetic field properties of NaNiO2

被引:0
作者
E. Chappel
M.D. Núñez-Regueiro
F. Dupont
G. Chouteau
C. Darie
A. Sulpice
机构
[1] Grenoble High Magnetic Field Laboratory,
[2] CNRS and MPI-FKF,undefined
[3] BP 166X,undefined
[4] 38042 Grenoble,undefined
[5] France,undefined
[6] Laboratoire de Cristallographie,undefined
[7] CNRS,undefined
[8] BP 166X,undefined
[9] 38042 Grenoble,undefined
[10] France,undefined
[11] Centre de Recherches sur les Très Basses Températures,undefined
[12] CNRS,undefined
[13] BP 166X,undefined
[14] 38042 Grenoble,undefined
[15] France,undefined
来源
The European Physical Journal B - Condensed Matter and Complex Systems | 2000年 / 17卷
关键词
PACS. 75.30.Et. Exchange and superexchange interactions - 76.50.+g Ferromagnetic, antiferromagnetic and ferrimagnetic resonances; spin-wave resonance;
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摘要
Magnetisation measurements up to 23 T and submillimeter wave ESR in the frequency region 48-380 GHz have been performed on NaNiO2 powders at low temperature. Also typical spectra above the Néel temperature \documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}\end{document} are shown. At 4 K the magnetisation shows a spin-flop transition at 1.8 T and saturation at 10 T. \documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}\end{document}/Ni confirms the low spin state of the Ni3+ ions. The susceptibility exhibits a maximum at \documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}\end{document} K with \documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}\end{document} and \documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}\end{document} K. NaNiO2 is an A-type antiferromagnet: we derive \documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}\end{document} K and \documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}\end{document} K for the interactions between Ni ions within and between adjacent layers, respectively. The AFMR spectra yield an energy gap of 52.5 GHz, in agreement with the spin-flop value derived from the magnetisation. The anisotropy of the g factor observed at 100 K with \documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}\end{document} can be attributed to the Jahn-Teller effect for Ni3+ ions in the low spin state, which stabilises the \documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}\end{document} occupation. We finally comment on the isomorphic controversial Li1-xNi1+xO2 compound.
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页码:609 / 614
页数:5
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