Molecules in a bicircular strong laser field

被引:0
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作者
Dino Habibović
Aner Čerkić
Mustafa Busuladžić
Azra Gazibegović-Busuladžić
Senad Odžak
Elvedin Hasović
Dejan B. Milošević
机构
[1] University of Sarajevo,Faculty of Science
[2] Max-Born-Institut,Faculty of Medicine
[3] University of Sarajevo,undefined
[4] Academy of Sciences and Arts of Bosnia and Herzegovina,undefined
来源
Optical and Quantum Electronics | 2018年 / 50卷
关键词
Improved molecular strong-field approximation; High-order above-threshold ionization; Reflection and rotational symmetry;
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摘要
Strong-field ionization of nonlinear planar triatomic molecules by a bicircular laser field is analyzed within the improved molecular strong-field approximation. Our calculations include additional interaction between the liberated electrons and atomic or ionic centers of the parent molecular ion. The used bicircular field consists of two counterrotating circularly polarized fields having angular frequencies rω\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$r \omega$$\end{document} and sω\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$s \omega$$\end{document}, with integer r and s. In the case when the laser-field-polarization plane is parallel to the plane of the considered molecule (example of ozone molecule is analyzed), the corresponding photoelectron spectra are not rotationally symmetric. On the other hand, when these planes are mutually perpendicular, for the (rω,sω)=(ω,3ω)\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$(r\omega ,s\omega )=(\omega ,3\omega )$$\end{document} bicircular field, the electron spectra satisfy the corresponding rotational symmetries. Analyzing the obtained spectra and the corresponding symmetries, one can extract information about molecular orientation and structure. This technique may also be useful for more complex polyatomic molecules.
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