Tuning metal-support interaction of Pt-based electrocatalysts for hydrogen energy conversion

被引：0
作者：
Shenzhou Li
Tanyuan Wang
Qing Li
机构：
[1] Huazhong University of Science and Technology,State Key Laboratory of Materials Processing and Die & Mould Technology, School of Materials Science and Engineering
[2] Shenzhen Huazhong University of Science and Technology Research Institute,undefined
来源：
Science China Chemistry | 2023年 / 66卷
关键词：
metal-support interaction; Pt-based catalysts; electrocatalysis; hydrogen evolution reaction; oxygen reduction reaction;
D O I：
暂无
中图分类号：
学科分类号：
摘要：
Pt-based electrocatalysts hold great promise for key electrocatalytic reactions in hydrogen-related energy conversion devices. Generally, the catalytic performance is significantly influenced by metal-support interactions (MSI) in the catalysts, making the tuning of MSI in Pt-based catalysts a highly intriguing research focus. In this review, the catalytic mechanism of Pt-based electrocatalysts is firstly introduced. Subsequently, the effects of MSI on supported Pt electrocatalysts are summarized into four types: geometric effects, electronic effects, synergistic effects, and structural reconfiguration. Finally, the prospect of optimizing the performance of Pt-based electrocatalysts by engineering MSI is exhibited, with the aim of inspiring innovation and advancement of supported Pt catalysts, thereby facilitating the development and utilization of hydrogen energy. [graphic not available: see fulltext]
引用
收藏
页码：3398 / 3414
页数：16
相关论文
共 1114 条
[1]  
Gasteiger HA(2009)undefined Science 324 48-49
[2]  
Marković NM(2012)undefined Nature 486 43-51
[3]  
Debe MK(2019)undefined Nat Catal 2 578-589
[4]  
Wang XX(2006)undefined Nat Mater 5 909-913
[5]  
Swihart MT(2015)undefined Chem Soc Rev 44 5148-5180
[6]  
Wu G(2013)undefined Nat Chem 5 300-306
[7]  
Greeley J(2010)undefined J Electrochem Soc 157 B1529-497
[8]  
Jaramillo TF(2007)undefined Science 315 493-2201
[9]  
Bonde J(2015)undefined Chem Soc Rev 44 2168-17892
[10]  
Chorkendorff I(2004)undefined J Phys Chem B 108 17886-13854
12345678910