Characteristics of colloids and their affinity for heavy metals in road runoff with different traffic in Beijing, China

被引:0
作者
Xiaoli Du
Hui Liang
Xing Fang
Shenshen Cui
Junqi Li
机构
[1] Beijing University of Civil Engineering and Architecture,Key Laboratory of Urban Stormwater System and Water Environment, Ministry of Education
[2] Beijing University of Civil Engineering and Architecture,Beijing Engineering Research Center of Sustainable Urban Sewage System Construction and Risk Control
[3] Auburn University,Department of Civil Engineering
来源
Environmental Science and Pollution Research | 2021年 / 28卷
关键词
Road runoff; Colloids; Traffic density; Heavy metals; Migration; Stability;
D O I
暂无
中图分类号
学科分类号
摘要
The characteristics of colloids in urban road runoff with different traffic in Beijing, China, such as concentration, particle size, chemical property, and affinity for heavy metals were determined. The concentration of colloids was high, and an evident first flush effect was found in the runoff of road with heavy traffic. A large portion of colloids were distributed in the range of 1–10 μm. Traffic activity, rainfall intensity, and time of sample collection would not change the size distribution of colloids in the road runoff. The chemical property of colloids in the road runoff would be influenced by the soil erosion nearby green space, causing the content of organic colloids was high. The correlation coefficient between the concentration of colloids in colloidal fractions and the concentration of heavy metals (Cu, Zn, Cd, Pb, Fe, and Mn) in the road runoff with different traffic decreased with the same sequence from 0.02–0.2 μm, 0.2–0.45 μm, 0.45–1 μm, to 1–10 μm, suggesting that the heavy metals had stronger affinity for the colloids with small size. The concentration of Cu, Pb, and Zn exhibited significant correlations with the concentration of organic colloids in the road runoff. More aggregated spherical particles were found in the TEM image of the road runoff with heavy traffic. Zeta potentials and RMV data showed that the colloids with smaller size and the colloids in the road runoff with lighter traffic were much more stable.
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页码:20082 / 20092
页数:10
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共 158 条
  • [11] Cantu A(2009)Temporal variability of colloidal material in agricultural storm runoff from managed grassland using flow field-flow fractionation J Chromatog A 1216 9120-9124
  • [12] Hood EM(2016)Colloidal mobilization of arsenic from mining-affected soils by surface runoff Chemosphere 144 1123-1131
  • [13] Coleman CH(2013)Partitioning of polycyclic aromatic hydrocarbons, alkylphenols, bisphenol A and phthalates in landfill leachates and stormwater Water Res 47 1317-1328
  • [14] Corapcioglu MO(2006)Subsurface transport of Cd, Cr, and Mo mediated by biosolid colloids Sci Total Environ 354 157-169
  • [15] Santschi PH(2010)Stability and aggregation of metal oxide nanoparticles in natural aqueous matrices Environ Sci Technol 44 1962-1967
  • [16] Brown J(2008)Reductive transformation of pentachlorophenol on the interface of subtropical soil colloids and water Geoderma 148 70-78
  • [17] Stein E(2019)Transport behavior of variable charge soil particle size fractions and their influence on cadmium transport in saturated porous media Geoderma 337 945-955
  • [18] Ackerman D(2009)Bioavailability and fate of phosphorus in constructed wetlands receiving agricultural runoff in the San Joaquin Valley, California J Environ Qual 38 360-372
  • [19] Dorsey J(2002)Influence of ionic strength and cation charge on transport of colloidal particles in fractured shale saprolite Environ Sci Technol 36 3735-3743
  • [20] Lyon J(2013)Effect of natural particles on the transport of lindane in saturated porous media: laboratory experiments and model-based analysis J Contam Hydrol 149 13-26