Synthesis and nonlinear optical susceptibility of cyanine dye J-aggregates doped silica film (II)

被引:22
|
作者
Zhou H.S. [1 ]
Watanabe T. [2 ]
Mito A. [3 ]
Asai K. [2 ]
Ishigure K. [2 ]
Honma I. [1 ]
机构
[1] Electrotechnical Laboratory, AIST, Umezono, Tsukuba
[2] Dept. of Quant. Eng. and Syst. Sci., University of Tokyo, Tokyo, 113, Hongo, Bunkyo-ku
[3] Natl. Res. Laboratory of Metrology, AIST, Umezono, Tsukuba
关键词
modified sol-gel; J-aggregates; nonlinear optical susceptibility; z-scan method;
D O I
10.1023/A:1008720402488
中图分类号
学科分类号
摘要
We tried to embed stable J-aggregates of 1,1′-diethyl-2,2′-cyanine bromide into a thin silica film by simple sol-gel processing. Its third order susceptibility |χ(3)| was about 5 × 10-7 esu at resonance wavelength of the J band by Z-scan method using a 180-femtosecond pulse laser beam at 77 K in vacuum environment (< 10-5 Torr). The net |χ(3)| value of pure J-aggregates should be 4 × 10-6 esu from the doping ration of J-aggregates in silica film.
引用
收藏
页码:803 / 806
页数:3
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