Vibrational dynamics in liquids studied by non-linear infrared spectroscopy

被引：0
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作者：
Hiroaki Maekawa
Kaoru Ohta
Keisuke Tominaga
机构：
来源：
Research on Chemical Intermediates | 2005年 / 31卷
关键词：
THREE-PULSE PHOTON ECHO; VIBRATIONAL DEPHASING; SOLVATION DYNAMICS; DI-P-TOLYLCARBODIIMIDE; NON-LINEAR INFRARED SPECTROSCOPY;
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摘要：
Three-pulse photon echo experiments in the infrared region have been performed to study vibrational dephasing and transition frequency fluctuations in solutions. Time-integrated and frequency-resolved photon echo signals of the –N=C=N– anti-symmetric stretching mode of di-p-tolylcarbodiimide show an oscillatory behavior due to interference with a band nearby. Solvation dynamics or frequency fluctuations of several ions in hydrogen-bonding solvents have been studied and a couple of general trends of the time-correlation function of the frequency fluctuation on these systems have been observed.
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页码：703 / 716
页数：13
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