Experimental determination of the diffusion coefficient in two-dimensions in ferrous sulphate gels using the finite element method

被引:99
作者
Baldock C. [1 ]
Harris P.J. [2 ]
Piercy A.R. [3 ]
Healy B. [4 ]
机构
[1] Ctr. for Medical and Health Physics, Queensland University of Technology, Brisbane
[2] School of Computing and Mathematical Sciences, University of Brighton
[3] School of Engineering, University of Brighton
[4] Queensland Radium Institute, Mater Hospital, Brisbane
来源
Australasian Physics & Engineering Sciences in Medicine | 2001年 / 24卷 / 1期
关键词
Diffusion Coefficient; Finite Element Method; Finite Difference Method; Glass Beaker; Drift Parameter;
D O I
10.1007/BF03178282
中图分类号
学科分类号
摘要
A novel two-dimensional finite element method for modelling the diffusion which occurs in Fricke or ferrous sulphate type radiation dosimetry gels is presented. In most of the previous work, the diffusion coefficient has been estimated using simple one-dimensional models. This work presents a two-dimensional model which enables the diffusion coefficient to be determined in a much wider range of experimental situations. The model includes the provision for the determination of a drift parameter. To demonstrate the technique comparative diffusion measurements between ferrous sulphate radiation dosimetry gels, with and without xylenol orange chelating agent and carbohydrate additives have been undertaken. Diffusion coefficients of 9.7±0.4, 13.3±0.6 and 9.5±0.8 10-3 cm2h-1 were determined for ferrous sulphate radiation dosimetry gels with and without xylenol orange and with xylenol orange and sucrose additives respectively.
引用
收藏
页码:19 / 30
页数:11
相关论文
共 32 条
[11]  
Harris P.J., Piercy A., Baldock C., A method for determining the diffusion coefficient in Fe(II/III) radiation dosimetry gels using finite elements, Phys. Med. Biol., 41, pp. 1745-1753, (1996)
[12]  
Rae W.I.D., Willemse C.A., Lotter M.G., Engelbrecht J.S., Swarts J.C., Chelator effect on ion diffusion in ferrous-sulfate-doped gelatin gel dosimeters as analyzed by MRI, Med. Phys., 23, pp. 15-23, (1996)
[13]  
Kron T., Jonas D., Pope J.M., Fast T-1 imaging of dual gel samples for diffusion measurements in NMR dosimetry gels, Magn. Reson. Imaging, 15, pp. 211-221, (1997)
[14]  
Pedersen T.V., Olsen D.R., Skretting A., Measurement of the ferric diffusion coefficient in agarose and gelatine gels by utilization of the evolution of a radiation induced edge as reflected in relaxation rate images, Phys. Med. Biol., 42, pp. 1575-1585, (1997)
[15]  
Schreiner L.J., Crooks I., Evans M.D.C., Keller B.M., Parker W.A., Imaging of HDR brachytherapy dose distributions using NMR Fricke-gelatin dosimetry, Magn. Reson. Imaging, 12, pp. 901-907, (1994)
[16]  
Chu W.C., Kao Y.H., Chung W.Y., Guo W.Y., Pan H.C., Ferric ion diffusion effects in NMR-Fricke-agarose dosimetry, Proceedings of International Society for Magnetic Resonance in Medicine, (1998)
[17]  
Chu K.C., Jordan K.J., Battista J.J., Van Dyk J., Rutt B.K., Polyvinyl alcohol-Fricke hydrogel and cryogel: Two new gel dosimetry systems with low Fe3+ diffusion, Phys. Med. Biol., 45, pp. 955-969, (2000)
[18]  
Clarke G.D., McColl R.W., Maryanski M.J., Glatstein E., Imaging of radiation dose in two different types of gel-based dosimeters: A comparison between FAX and BANG, Med. Phys., 22, (1995)
[19]  
Olsson L.E., (1991)
[20]  
Zahmatkesh M., (1999)