Model Evaluation of Indoor Exposure to Polychlorinated Dibenzo-p-Dioxins and Dibenzofurans and Polycyclic Aromatic Hydrocarbons from Household Fuel Combustion in Rural Areas of Tibetan Plateau

被引:0
作者
Rong Jin
Minghui Zheng
Lili Yang
Gerhard Lammel
Xin Zhou
Yuxiang Sun
Changzhi Chen
Bingcheng Lin
Guorui Liu
机构
[1] Hangzhou Institute for Advanced Study,School of Environment
[2] University of Chinese Academy of Sciences,State Key Laboratory of Environmental Chemistry and Ecotoxicology
[3] Research Center for Eco-Environmental Sciences,College of Resources and Environment
[4] Chinese Academy of Sciences,Faculty of Science
[5] University of Chinese Academy of Sciences,Zhejiang Key Laboratory of Ecological and Environmental Monitoring, Forewarning and Quality Control
[6] Multiphase Chemistry Department,undefined
[7] Max Planck Institute for Chemistry,undefined
[8] RECETOX,undefined
[9] Masaryk University,undefined
[10] Zhejiang Ecological and Environmental Monitoring Center,undefined
来源
Exposure and Health | 2023年 / 15卷
关键词
Tibetan Plateau; Herdsman; Indoor air pollution; Persistent organic pollutant; Dioxin; Health risk;
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中图分类号
学科分类号
摘要
Polychlorinated dibenzo-p-dioxins and dibenzofurans (PCDD/Fs) and polycyclic aromatic hydrocarbons (PAHs) are toxic pollutants produced by incomplete combustion. Household fuel combustion in rural homes is an understudied and potentially highly exposing source. We constructed a model of indoor exposure of Tibetan herdsmen and villagers to PCDD/Fs and PAHs, evaluated against measurements. Indoor PCDD/F concentrations for herdsmen and villagers are predicted to be 198–8912 and 313–5700 fg m−3 (95% confidence interval [CI]), respectively. For PAHs, these ranges are 793–9483 and 509–5497 ng m−3 (95% CI), respectively. The PCDD/F values are higher than those encountered in ambient air of Beijing on haze days. Daily intakes of PCDD/Fs for children (4.17–111 fg toxic equivalent (TEQ) d−1 kg–1) were higher than those for adolescents (1.88–50.0 fg TEQ d−1 kg−1) and adults (1.63–43.4 fg TEQ d−1 kg−1). Cancer risks associated with PCDD/F exposure for rural Tibetan residents ([0.18–7.08] × 10−5 for herdsmen and [0.36–4.92] × 10−5 for villagers; 95% CI) were similar to those for workers in metallurgical plants ([1.44–4.19] × 10−5). The family income and lifestyle were identified as key factors influencing household fuel use. Rural Tibetans are exposed to indoor POP pollution produced by household fuel combustion and the risks associated with this should be mitigated.
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页码:145 / 159
页数:14
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