Exploring the capture and desorption of CO2 on graphene oxide foams supported by computational calculations

被引:13
作者
Hoyos, Bryan E. Arango [1 ]
Osorio, H. Franco [2 ]
Gomez, E. K. Valencia [3 ]
Sanchez, J. Guerrero [4 ]
Palominos, A. P. Del Canto [1 ]
Larrain, Felipe A. [1 ]
Barragan, J. J. Prias [2 ,3 ]
机构
[1] Univ Adolfo Ibanez, Fac Engn & Sci, Energy Engn, Santiago 7941169, Chile
[2] Univ Quindio, Fac Basic Sci & Technol, Elect Instrumentat Technol Program, Armenia 630001, Colombia
[3] Univ Quindio, Interdisciplinary Inst Sci, Doctoral Program Phys Sci, Armenia 630004, Colombia
[4] Univ Nacl Autonoma Mexico, Ctr Nanosci & Nanotechnol, Virtual Mat Modeling Lab LVMM, Ensenada 22860, Mexico
关键词
CARBON-DIOXIDE; AB-INITIO; FLUE-GAS; ADSORPTION; AIR; SEPARATION; SILICA; ADSORBENT; EXTRACTION; SORBENTS;
D O I
10.1038/s41598-023-41683-4
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
In the last decade, the highest levels of greenhouse gases (GHG) in the atmosphere have been recorded, with carbon dioxide (CO2) being one of the GHGs that most concerns mankind due to the rate at which it is generated on the planet. Given its long time of permanence in the atmosphere (between 100 to 150 years); this has deployed research in the scientific field focused on the absorption and desorption of CO2 in the atmosphere. This work presents the study of CO2 adsorption employing materials based on graphene oxide (GO), such as GO foams with different oxidation percentages (3.00%, 5.25%, and 9.00%) in their structure, obtained via an environmentally friendly method. The characterization of CO2 adsorption was carried out in a closed system, within which were placed the GO foams and other CO2 adsorbent materials (zeolite and silica gel). Through a controlled chemical reaction, production of CO2 was conducted to obtain CO2 concentration curves inside the system and calculate from these the efficiency, obtained between 86.28 and 92.20%, yield between 60.10 and 99.50%, and effectiveness of CO2 adsorption of the materials under study. The results obtained suggest that GO foams are a promising material for carbon capture and the future development of a new clean technology, given their highest CO2 adsorption efficiency and yield.
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收藏
页数:15
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