Preparation of hollow spherical covalent organic frameworks via Oswald ripening under ambient conditions for immobilizing enzymes with improved catalytic performance

被引:0
作者
Hao Zhao
Guanhua Liu
Yunting Liu
Liya Zhou
Li Ma
Ying He
Xiaobing Zheng
Jing Gao
Yanjun Jiang
机构
[1] Hebei University of Technology,School of Chemical Engineering and Technology
[2] Hubei University,State Key Laboratory of Biocatalysis and Enzyme Engineering, School of Life Sciences
来源
Nano Research | 2023年 / 16卷
关键词
hollow spherical structure; covalent organic framework; Oswald ripening mechanism; lipase; kinetic resolution;
D O I
暂无
中图分类号
学科分类号
摘要
The hollow spherical covalent organic frameworks (COFs) have a wide application prospect thanks to their special structures. However, the controllable synthesis of uniform and stable hollow COFs is still a challenge. We herein propose a self-templated method for the preparation of hollow COFs through the Ostwald ripening mechanism under ambient conditions, which avoids most disadvantages of the commonly used hard-templating and soft-templating methods. A detailed time-dependent study reveals that the COFs are transformed from initial spheres to hollow spheres because of the inside-out Ostwald ripening process. The obtained hollow spherical COFs have high crystallinity, specific surface area (2,036 m2·g−1), stability, and single-batch yield. Thanks to unique hollow structure, clear through holes, and hydrophobic pore environment of the hollow spherical COFs, the obtained immobilized lipase (BCL@H-COF-OMe) exhibits higher thermostability, polar organic solvent tolerance, and reusability. The BCL@H-COF-OMe also shows higher catalytic performance than the lipase immobilized on non-hollow COF and free lipase in the kinetic resolution of secondary alcohols. This study provides a simple approach for the preparation of hollow spherical COFs, and will promote the valuable research of COFs in the field of biocatalysis.
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页码:281 / 289
页数:8
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