An experimental study on the simultaneous removal of NO and SO2 with a new wet recycling process based on the micro-nano bubble water system

被引:0
作者
Zhengguo Xiao
Dengxin Li
Rongliang Zhang
Feikun Wang
Fanfeng Pan
Zhihong Sun
机构
[1] Donghua University,College of Environmental Science and Engineering
[2] Tongji University,State Key Laboratory of Pollution Control and Resource Reuse, College of Environmental Science and Engineering
[3] China New Energy (Shanghai) Limited Company,undefined
来源
Environmental Science and Pollution Research | 2020年 / 27卷
关键词
Wet process; NO; SO; Desulfurization; Denitration; Micro-nano bubble;
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摘要
The micronano bubble water system (MNBW) generated by a micronano bubble generator (MNBG) has the superior oxidation properties and can improve gas solubility. In the study, a new wet recycling process based on MNBW is proposed to simultaneously remove nitric oxide (NO) and sulfur dioxide (SO2). The important experimental parameters such as initial water pH, initial water temperature, NO and SO2 concentrations, and the presence of oxygen (O2) were investigated to explore the feasibility of desulfurization and denitration with MNBW. The experimental results showed that decreasing initial water pH or increasing initial water temperature and NO and SO2 concentrations were not conducive to the removal of NO or SO2. O2 could promote the removal of NO, but it had no effect on SO2 removal. In addition, SO2 removal efficiency always remained high and did not change obviously during the experimental period. However, NO removal efficiency gradually decreased in the first 50 min and then became stable.
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页码:4197 / 4205
页数:8
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  • [1] Adewuyi YG(2002)Sonochemical oxidation of carbon disulfide in aqueous solutions: reaction kinetics and pathways Ind Eng Chem Res 41 4957-4964
  • [2] Appaw C(2012)Modeling the ultrasonic cavitation-enhanced removal of nitrogen oxide in a bubble column reactor AICHE J 58 2397-2411
  • [3] Adewuyi YG(2006)Ultrasound-induced aqueous removal of nitric oxide from flue gases: effects of sulfur dioxide, chloride, and chemical oxidant J Phys Chem A 110 11098-11107
  • [4] Khan NE(2013)Simultaneous absorption and oxidation of nitric oxide and sulfur dioxide by aqueous solutions of sodium persulfate activated by temperature Ind Eng Chem Res 52 11702-11711
  • [5] Adewuyi YG(1984)The effect of pH on the conversion of superoxide to hydroxyl free radicals Arch Biochem Biophys 234 258-264
  • [6] Owusu SO(2002)ECO demonstrates the attractions of multipollutant control Mod Power Syst 5 39-43
  • [7] Adewuyi YG(2012)Structure of the nanobubble clusters of dissolved air in liquid media J Biol Phys 38 121-152
  • [8] Sakyi NY(1988)Rate constants for reactions of radicals in aqueous solution J Phys Chem 17 513-886
  • [9] Baker MS(1993)Removal of SO J Environ Eng 119 414-423
  • [10] Gebicki JM(2011) and NO from gas streams with combined plasma photolysis J Photochem Photobiol A 222 70-76