S-matrix theory of high harmonic generation and ionization of coherently ro-vibrating linear molecules by intense ultrashort laser pulses

被引:0
作者
F. H. M. Faisal
机构
[1] Universität Bielefeld,Fakultät für Physik
来源
Theoretical Chemistry Accounts | 2010年 / 127卷
关键词
S-Matrix theory; High harmonic generation,; Ionization; Ro-vibration; Intense; Ultrashort; Laser pulses; Pump-prove signal; Time-delay; Clock-motion;
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学科分类号
摘要
A theory of high harmonic generation and ionization of coherently rotating and vibrating linear molecules by a delayed pair of intense ultrashort laser pulses is presented. It correlates the nuclear motions in real time with the modulation of the harmonic emission and ionization signals as a function of the time-delay between the exciting and the probing pulses. An illustrative analytical example of the excitation and detection of the clock-motion associated with the “0–1” vibrational oscillation of a diatomic molecule is also given.
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页码:175 / 182
页数:7
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