Excitons in strain-induced one-dimensional moiré potentials at transition metal dichalcogenide heterojunctions

被引:0
作者
Yusong Bai
Lin Zhou
Jue Wang
Wenjing Wu
Leo J. McGilly
Dorri Halbertal
Chiu Fan Bowen Lo
Fang Liu
Jenny Ardelean
Pasqual Rivera
Nathan R. Finney
Xu-Chen Yang
D. N. Basov
Wang Yao
Xiaodong Xu
James Hone
Abhay N. Pasupathy
X.-Y. Zhu
机构
[1] Columbia University,Department of Chemistry
[2] Nanjing University,College of Engineering and Applied Sciences
[3] Columbia University,Department of Physics
[4] Columbia University,Department of Mechanical Engineering
[5] University of Washington,Department of Physics and Department of Materials Science and Engineering
[6] University of Hong Kong,Department of Physics
来源
Nature Materials | 2020年 / 19卷
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摘要
The possibility of confining interlayer excitons in interfacial moiré patterns has recently gained attention as a strategy to form ordered arrays of zero-dimensional quantum emitters and topological superlattices in transition metal dichalcogenide heterostructures. Strain is expected to play an important role in the modulation of the moiré potential landscape, tuning the array of quantum dot-like zero-dimensional traps into parallel stripes of one-dimensional quantum wires. Here, we present real-space imaging of unstrained zero-dimensional and strain-induced one-dimensional moiré patterns along with photoluminescence measurements of the corresponding excitonic emission from WSe2/MoSe2 heterobilayers. Whereas excitons in zero-dimensional moiré traps display quantum emitter-like sharp photoluminescence peaks with circular polarization, the photoluminescence emission from excitons in one-dimensional moiré potentials shows linear polarization and two orders of magnitude higher intensity. These results establish strain engineering as an effective method to tailor moiré potentials and their optoelectronic response on demand.
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页码:1068 / 1073
页数:5
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