Efficient blue light-emitting diodes based on quantum-confined bromide perovskite nanostructures

被引:1
作者
Yang Liu
Jieyuan Cui
Kai Du
He Tian
Zhuofei He
Qiaohui Zhou
Zhaoliang Yang
Yunzhou Deng
Dong Chen
Xiaobing Zuo
Yang Ren
Liang Wang
Haiming Zhu
Baodan Zhao
Dawei Di
Jianpu Wang
Richard H. Friend
Yizheng Jin
机构
[1] Zhejiang University,Centre for Chemistry of High
[2] Zhejiang University,Performance & Novel Materials, State Key Laboratory of Silicon Materials, School of Materials Science and Engineering
[3] Zhejiang University,Centre for Chemistry of High
[4] Zhejiang University,Performance & Novel Materials, State Key Laboratory of Silicon Materials, Department of Chemistry
[5] X-Ray Science Division,Centre of Electron Microscope, State Key Laboratory of Silicon Material, School of Material Science and Engineering
[6] Argonne National Laboratory,Center of Chemistry of High
[7] Beijing Institute of Technology,Performace & Novel Materials, Department of Chemistry
[8] University of Cambridge,School of Materials Science and Engineering
[9] Zhejiang University,Cavendish Laboratory
[10] Nanjing Tech University (NanjingTech),State Key Laboratory of Modern Optical Instrumentation, College of Optical Science and Engineering
来源
Nature Photonics | 2019年 / 13卷
关键词
D O I
暂无
中图分类号
学科分类号
摘要
The emergence of inorganic–organic hybrid perovskites, a unique class of solution-processable crystalline semiconductors, provides new opportunities for large-area, low-cost and colour-saturated light-emitting diodes (LEDs) ideal for display and solid-state lighting applications1. However, the performance of blue perovskite LEDs (PeLEDs)2–11 is far inferior to that of their near-infrared, red and green counterparts12–19, strongly limiting the practicality of the PeLED technology. Here, we demonstrate blue PeLEDs emitting at 483 nm with colour coordinates of (0.094, 0.184) and operating with a peak external quantum efficiency of up to 9.5% at a luminance of 54 cd m–2. The devices have a T50 lifetime of 250 s for an initial brightness of 100 cd m–2. The efficient blue electroluminescence originates from a structure of quantum-confined perovskite nanoparticles embedded within quasi-two-dimensional phases with higher bandgaps, prepared by an antisolvent processing scheme. Our work paves the way towards high-performance PeLEDs in the blue region.
引用
收藏
页码:760 / 764
页数:4
相关论文
共 66 条
[1]  
Tan ZK(2014)Bright light-emitting diodes based on organometal halide perovskite Nat. Nanotechnol. 9 687-692
[2]  
Song J(2015)Quantum dot light-emitting diodes based on inorganic perovskite cesium lead halides (CsPbX Adv. Mater. 27 7162-7167
[3]  
Li G(2016)) Adv. Mater. 28 3528-3534
[4]  
Pan J(2016)Highly efficient perovskite nanocrystal light-emitting diodes enabled by a universal crosslinking method Adv. Mater. 28 8718-8725
[5]  
Chen Z(2017)Highly efficient perovskite-quantum-dot light-emitting diodes by surface engineering Adv. Mater. 29 1603157-29906
[6]  
Yao EP(2017)High-performance color-tunable perovskite light emitting devices through structural modulation from bulk to layered film Adv. Mater. 29 1606859-2433
[7]  
Wang Q(2017)High-brightness blue and white LEDs based on inorganic perovskite nanocrystals and their composites ACS Appl. Mater. Interfaces 9 29901-242
[8]  
Ren J(2018)Efficient sky-blue perovskite light-emitting devices based on ethylammonium bromide induced layered perovskites Adv. Mater. 30 1706226-1225
[9]  
Peng XF(2018)Reducing architecture limitations for efficient blue perovskite light-emitting diodes Joule 2 2421-877
[10]  
Ji XX(2018)Efficient blue and white perovskite light-emitting diodes via manganese doping Nat. Commun. 9 235-704