Meteorological factors contributing to organic and elemental carbon concentrations in PM10 near an open-pit coal mine

被引:0
作者
Heli A. Arregocés
Roberto Rojano
Gloria Restrepo
机构
[1] Universidad de La Guajira,Grupo de Investigación GISA, Facultad de Ingeniería
[2] Universidad de Antioquia SIU/UdeA,Grupo Procesos Fisicoquímicos Aplicados, Facultad de Ingeniería
来源
Environmental Science and Pollution Research | 2022年 / 29卷
关键词
Biomass burning; Carbonaceous aerosols; Coal; Elemental carbon; Open-pit mining; Organic carbon;
D O I
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中图分类号
学科分类号
摘要
Variations in the carbonaceous aerosol contents, organic carbon (OC) and elemental carbon (EC), in particulate matter less than 10 μm in size (PM10), were analyzed at sites influenced by coal mining in an open-pit mine located in northern Colombia. Samples were collected during different seasonal periods throughout 2015. Meteorological variables for each site were examined during the different seasons. Aerosols were detected using a thermal-optical reflectance protocol method. The highest PM10 concentrations, between the ranges of 28.2 ± 8.2 μg m−3 and 75.0 ± 36.5 μg m−3, were recorded during the dry season. However, the highest concentrations of OC (4.8–14.2 μg m−3) and EC (2.9–13.9 μg m−3) in PM10 were observed during the transition period between the dry and wet seasons. The strong correlation between OC and EC in PM10 (r = 0.6–1.0) during the transition season indicates a common primary combustion source. High OC (> 8.3 μg m−3) and EC (> 6.9 μg m−3) concentrations were associated with low wind speeds (< 2.1 m s−1) moving in different directions. Analyses of the sources of atmospheric aerosol pollutants in the mining area in northern Colombia showed that the daily maximum total carbon concentrations were mainly associated with regional atmospheric transport of particulate matter from industrial areas and biomass burning sites located in the territory of Venezuela.
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页码:28854 / 28865
页数:11
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  • [1] Aamaas B(2011)Elemental carbon deposition to Svalbard snow from Norwegian settlements and long-range transport Tellus Ser B Chem Phys Meteorol 63 340-351
  • [2] Bøggild CE(2019)A systematic review on global pollution status of particulate matter-associated potential toxic elements and health perspectives in urban environment Environ Geochem Health 41 1131-1162
  • [3] Stordal F(1997)Atmospheric aerosols: biogeochemical sources and role in atmospheric chemistry Science (80- ) 276 1052-1058
  • [4] Ali MU(2017)Changing patterns of fire occurrence in proximity to forest edges, roads and rivers between NW Amazonian countries Biogeosciences 14 2755-2765
  • [5] Liu G(2020)Characteristics of carbonaceous matter in aerosol from selected urban and rural areas of Southern Poland Atmosphere (Basel) 11 687-1051
  • [6] Yousaf B(2008)Ambient site, home outdoor and home indoor particulate concentrations as proxies of personal exposures J Environ Monit 10 1041-4456
  • [7] Andreae MO(2004)Spatial and seasonal variations of atmospheric organic carbon and elemental carbon in Pearl River Delta Region, China Atmos Environ 38 4447-3137
  • [8] Armenteras D(2005)Characterization and source apportionment of atmospheric organic and elemental carbon during fall and winter of 2003 in Xi’an, China Atmos Chem Phys 5 3127-380
  • [9] Barreto JS(2017)Chemical characteristics of PM2. 5 during a 2016 winter haze episode in Shijiazhuang, China Aerosol Air Qual Res 17 368-4422
  • [10] Tabor K(2004)Equivalence of elemental carbon by thermal/optical reflectance and transmittance with different temperature protocols Environ Sci Technol 38 4414-1023