Aromatic ring substituted g-C3N4 for enhanced photocatalytic hydrogen evolution

被引:115
作者
Yu, Yu [1 ]
Yan, Wei [1 ]
Gao, Wenyu [1 ]
Li, Pei [1 ]
Wang, Xiaofang [1 ]
Wu, Songmei [1 ]
Song, Weiguo [2 ]
Ding, Kejian [1 ]
机构
[1] Beijing Jiaotong Univ, Sch Sci, Beijing 100044, Peoples R China
[2] Chinese Acad Sci, Inst Chem, Beijing 100190, Peoples R China
基金
中国国家自然科学基金;
关键词
CARBON NITRIDE NANOSHEETS; ELECTRONIC-STRUCTURE; GRAPHITIC C3N4; LIGHT; SEMICONDUCTORS; SEPARATION; CATALYSTS; TRIAZINE; WATER;
D O I
10.1039/c7ta05744j
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A facile strategy to fabricatemodified g-C3N4 with all-carbon aromatic rings incorporated in the constitutive plane was presented. The light absorption, band structure and photo-induced carrier separation of this benzene doped g-C3N4 was extremely improved. It exhibited a 3 times higher hydrogen evolution rate (HER) and a 17 times higher HER per surface area.
引用
收藏
页码:17199 / 17203
页数:5
相关论文
共 42 条
[1]  
[Anonymous], 2016, ANGEW CHEM INT EDIT
[2]   FT-IR/PA STUDY OF QUINOLINE ADSORBED ON CALCINED AND SULFIDED MO/GAMMA-AL2O3 [J].
BANDYOPADHYAY, S ;
MASSOTH, FE ;
PONS, S ;
EYRING, EM .
JOURNAL OF PHYSICAL CHEMISTRY, 1985, 89 (12) :2560-2564
[3]   Harvesting Solar Light with Crystalline Carbon Nitrides for Efficient Photocatalytic Hydrogen Evolution [J].
Bhunia, Manas K. ;
Yamauchi, Kazuo ;
Takanabe, Kazuhiro .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2014, 53 (41) :11001-11005
[4]   A JOINT THEORETICAL AND EXPERIMENTAL-STUDY OF THE ALUMINUM POLYETHYLENE TEREPHTHALATE INTERFACE [J].
CALDERONE, A ;
LAZZARONI, R ;
BREDAS, JL ;
LE, QT ;
PIREAUX, JJ .
SYNTHETIC METALS, 1994, 67 (1-3) :97-101
[5]   Construction of Graphitic C3N4-Based Intramolecular Donor - Acceptor Conjugated Copolymers for Photocatalytic Hydrogen Evolution [J].
Fan, Xiangqian ;
Zhang, Lingxia ;
Cheng, Ruolin ;
Wang, Min ;
Li, Mengli ;
Zhou, Yajun ;
Shi, Jianlin .
ACS CATALYSIS, 2015, 5 (09) :5008-5015
[6]   In situ synthesis of graphitic-C3N4 nanosheet hybridized N-doped TiO2 nanofibers for efficient photocatalytic H2 production and degradation [J].
Han, Cheng ;
Wang, Yingde ;
Lei, Yongpeng ;
Wang, Bing ;
Wu, Nan ;
Shi, Qi ;
Li, Qiong .
NANO RESEARCH, 2015, 8 (04) :1199-1209
[7]   Atomically Thin Mesoporous Nanomesh of Graphitic C3N4 for High-Efficiency Photocatalytic Hydrogen Evolution [J].
Han, Qing ;
Wang, Bing ;
Gao, Jian ;
Cheng, Zhihua ;
Zhao, Yang ;
Zhang, Zhipan ;
Qu, Liangti .
ACS NANO, 2016, 10 (02) :2745-2751
[8]   A Graphitic-C3N4 "Seaweed" Architecture for Enhanced Hydrogen Evolution [J].
Han, Qing ;
Wang, Bing ;
Zhao, Yang ;
Hu, Chuangang ;
Qu, Liangti .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2015, 54 (39) :11433-11437
[9]   Hybrid functionals based on a screened Coulomb potential [J].
Heyd, J ;
Scuseria, GE ;
Ernzerhof, M .
JOURNAL OF CHEMICAL PHYSICS, 2003, 118 (18) :8207-8215
[10]   Carbon nitride with simultaneous porous network and O-doping for efficient solar-energy-driven hydrogen evolution [J].
Huang, Zhen-Feng ;
Song, Jiajia ;
Pan, Lun ;
Wang, Ziming ;
Zhang, Xueqiang ;
Zou, Ji-Jun ;
Mi, Wenbo ;
Zhang, Xiangwen ;
Wang, Li .
NANO ENERGY, 2015, 12 :646-656