Liquid phase therapy to solid electrolyte-electrode interface in solid-state Li metal batteries: A review

被引：248

作者：

Zhao, Chen-Zi ^{[1
]}

Zhao, Bo-Chen ^{[1
]}

Yan, Chong ^{[2
]}

Zhang, Xue-Qiang ^{[1
]}

Huang, Jia-Qi ^{[2
]}

Mo, Yifei ^{[3
]}

Xu, Xiaoxiong ^{[4
]}

Li, Hong ^{[5
]}

Zhang, Qiang ^{[1
]}

机构：

[1] Tsinghua Univ, Beijing Key Lab Green Chem React Engn & Technol, Dept Chem Engn, Beijing 100084, Peoples R China

[2] Beijing Inst Technol, Adv Res Inst Multidisciplinary Sci, Beijing 100081, Peoples R China

[3] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA

[4] Chinese Acad Sci, Ningbo Inst Mat Technol & Engn, Ningbo 315201, Zhejiang, Peoples R China

[5] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China

来源：

ENERGY STORAGE MATERIALS | 2020年 / 24卷 / 24期

基金：

中国国家自然科学基金;

关键词：

Solid-state rechargeable batteries; Electrolyte-electrode interface; Lithium metal anode; Liquid electrolyte; Solid electrolyte interface; LITHIUM-ION TRANSFER; HYBRID ELECTROLYTES; POLYMER ELECTROLYTES; INTERPHASE FORMATION; CERAMIC ELECTROLYTE; CHEMICAL-STABILITY; SULFUR BATTERIES; RATE CAPABILITY; LI10GEP2S12; CHALLENGES;

D O I：

10.1016/j.ensm.2019.07.026

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Solid-state lithium (Li) metal batteries, employing solid electrolytes, with high energy density and enhanced safety are promising choices for next-generation electrochemical energy storage devices. However, the large interfacial resistances seriously hinder their commercialization. To construct a conformal interface with acceptable resistances, introducing small amounts of additional liquid electrolytes is one of the most convenient and effective solutions. This review summarizes the fundamental understandings on the interfacial behaviors between liquid electrolytes, electrodes and solid-state electrolytes. Afterwards, emerging strategies are discussed, involving interfacial wetting, in situ polymerization and interfacial reactions. Finally, current limitations and perspectives are presented for liquid phase therapy regarding the interfacial science and engineering.

引用

页码：75 / 84

页数：10

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