Impact of combustion phase on scattering and spectral absorption of Siberian biomass burning: studies in Large Aerosol Chamber

被引:3
作者
Popovicheva, O. B. [1 ]
Kozlov, V. S. [2 ]
机构
[1] Moscow MV Lomonosov State Univ, Skobelsyn Inst Nucl Phys, Moscow, Russia
[2] Zuev Inst Atmospher Opt RAS, Tomsk, Russia
来源
26TH INTERNATIONAL SYMPOSIUM ON ATMOSPHERIC AND OCEAN OPTICS, ATMOSPHERIC PHYSICS | 2020年 / 11560卷
关键词
Biomass burning; flaming; smoldering; scattering; absorption; MICROPHYSICAL PROPERTIES; SMOKE; CARBON; BOREAL; SIZE; EMISSIONS;
D O I
10.1117/12.2575583
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
Impact of Siberian biomass burning phase on optical properties of smoke aerosols is investigated in small-scale fires performed in a Large Aerosol Chamber (LAC). The analyses have revealed the influence of combustion temperature on scattering and light absorption of pine and debris smoke. Scattering in smoldering phase is significantly exceeding the flaming one. Spectral absorption obtained throughout the near-ultraviolet to near-infrared spectral region emphasizes the high absorption Angstrom exponent (AAE), up to 4.4 for fresh debris smoke, and a large fraction of light-absorbing brown carbon (BrC) in the smoldering phase. In opposite, open flaming smoke shows low AAE around 1, typical for high-temperature fossil fuel combustion while mixed fires emit particles absorbing with the intermediate AAE characteristics.
引用
收藏
页数:7
相关论文
共 28 条
[1]   Brown carbon spheres in East Asian outflow and their optical properties [J].
Alexander, Duncan T. L. ;
Crozier, Peter A. ;
Anderson, James R. .
SCIENCE, 2008, 321 (5890) :833-836
[2]   Organic tracers in aerosols from the residential combustion of pellets and agro-fuels [J].
Alves, Celia A. ;
Vicente, Estela D. ;
Rocha, Sonia ;
Vicente, Ana M. .
AIR QUALITY ATMOSPHERE AND HEALTH, 2017, 10 (01) :37-45
[3]   The size- and time-resolved composition of aerosols from a sub-Arctic boreal forest prescribed burn [J].
Cahill, Catherine F. ;
Cahill, Thomas A. ;
Perry, Kevin D. .
ATMOSPHERIC ENVIRONMENT, 2008, 42 (32) :7553-7559
[4]   Brown carbon aerosols from burning of boreal peatlands: microphysical properties, emission factors, and implications for direct radiative forcing [J].
Chakrabarty, Rajan K. ;
Gyawali, Madhu ;
Yatavelli, Reddy L. N. ;
Pandey, Apoorva ;
Watts, Adam C. ;
Knue, Joseph ;
Chen, Lung-Wen A. ;
Pattison, Robert R. ;
Tsibart, Anna ;
Samburova, Vera ;
Moosmuller, Hans .
ATMOSPHERIC CHEMISTRY AND PHYSICS, 2016, 16 (05) :3033-3040
[5]   Annual Variability of Black Carbon Concentrations Originating from Biomass and Fossil Fuel Combustion for the Suburban Aerosol in Athens, Greece [J].
Diapouli, Evangelia ;
Kalogridis, Athina-Cerise ;
Markantonaki, Christina ;
Vratolis, Stergios ;
Fetfatzis, Prodromos ;
Colombi, Cristina ;
Eleftheriadis, Konstantinos .
ATMOSPHERE, 2017, 8 (12)
[6]   Atmospheric Brown Clouds: From Local Air Pollution to Climate Change [J].
Engling, Guenter ;
Gelencser, Andras .
ELEMENTS, 2010, 6 (04) :223-228
[7]   Study of the competing chemical reactions in the initiation and spread of smouldering combustion in peat [J].
Hadden, Rory M. ;
Rein, Guillermo ;
Belcher, Claire M. .
PROCEEDINGS OF THE COMBUSTION INSTITUTE, 2013, 34 :2547-2553
[8]   Ambient measurements and source apportionment of fossil fuel and biomass burning black carbon in Ontario [J].
Healy, R. M. ;
Sofowote, U. ;
Su, Y. ;
Debosz, J. ;
Noble, M. ;
Jeong, C. -H. ;
Wang, J. M. ;
Hilker, N. ;
Evans, G. J. ;
Doerksen, G. ;
Jones, K. ;
Munoz, A. .
ATMOSPHERIC ENVIRONMENT, 2017, 161 :34-47
[9]   Correlations between optical, chemical and physical properties of biomass burn aerosols [J].
Hopkins, R. J. ;
Lewis, K. ;
Desyaterik, Y. ;
Wang, Z. ;
Tivanski, A. V. ;
Arnott, W. P. ;
Laskin, A. ;
Gilles, M. K. .
GEOPHYSICAL RESEARCH LETTERS, 2007, 34 (18)
[10]   Source characterization of biomass burning particles:: The combustion of selected European conifers, African hardwood, savanna grass, and German and Indonesian peat [J].
Iinuma, Y. ;
Brueggemann, E. ;
Gnauk, T. ;
Mueller, K. ;
Andreae, M. O. ;
Helas, G. ;
Parmar, R. ;
Herrmann, H. .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2007, 112 (D8)