Aqueous-phase hydrogenation of biomass-derived itaconic acid to methyl-γ-butyrolactone over Pd/C catalysts: Effect of pretreatments of active carbon

被引：16

作者：

Li, Sha ^{[1
,2
]}

Wang, Xicheng ^{[2
]}

Liu, Xiaoran ^{[2
]}

Xu, Guoqiang ^{[2
]}

Han, Sheng ^{[1
]}

Mu, Xindong ^{[2
]}

机构：

[1] Shanghai Inst Technol, Sch Chem & Environm Engn, Shanghai 201418, Peoples R China

[2] Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Key Lab Biobased Mat, Qingdao 266101, Peoples R China

来源：

CATALYSIS COMMUNICATIONS | 2015年 / 61卷

基金：

中国国家自然科学基金;

关键词：

Biomass; Itaconic acid; Methyl-gamma-butyrolactone; Hydrogenation; Pd/C; SUCCINIC ACID; PLATFORM CHEMICALS; LEVULINIC ACID; VALEROLACTONE; CONVERSION; 1,4-BUTANEDIOL; NANOPARTICLES; ELECTRODES; BIO;

D O I：

10.1016/j.catcom.2014.12.017

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

The effect of active carbon pretreatment on the catalytic performance of Pd/C catalysts in the hydrogenation of itaconic acid was studied. The catalysts were prepared by deposition-precipitation and characterized by XRD, BET, NH3-TPD, TEM and FT-IR. Due to the modification of the surface functional groups, surface structure and surface acidities of active carbon via pretreatment, the Pd/C catalysts showed varied catalytic performances. High dispersion and uniform particles were conducive to the excellent activity of Pd/C catalyst with support copretreated with HNO3 and NaClO, which exhibited 89.5% selectivity towards methyl-gamma-butyrolactone at 180 degrees C, 4 MPa H-2 for 20 h. (C) 2014 Elsevier B.V. All rights reserved.

引用

页码：92 / 96

页数：5

共 26 条

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