Plasmon damping below the Landau regime: the role of defects in epitaxial graphene

被引:67
作者
Langer, T. [1 ,2 ]
Baringhaus, J. [1 ]
Pfnuer, H. [1 ]
Schumacher, H. W. [2 ]
Tegenkamp, C. [1 ]
机构
[1] Leibniz Univ Hannover, Inst Festkorperphys, D-30167 Hannover, Germany
[2] Phys Tech Bundesanstalt, D-38116 Braunschweig, Germany
关键词
ENERGY BANDGAP; LAYERS; GRAPHITIZATION; DIFFRACTION; DISPERSION; GROWTH; ORIGIN;
D O I
10.1088/1367-2630/12/3/033017
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The sheet plasmon in epitaxially grown graphene layers on SiC(0001) and the influence of surface roughness have been investigated in detail by means of low-energy electron diffraction (LEED) and electron energy loss spectroscopy (EELS). We show that the existence of steps or grain boundaries in this epitaxial system is a source of strong damping, while the dispersion is rather insensitive to defects. To the first order, the lifetime of the plasmons was found to be proportional to the average terrace length and to the plasmon wavelength. A possible reason for this surprisingly efficient plasmon damping may be the close coincidence of phase (and group) velocities of the plasmons ( almost linear dispersion) with the Fermi velocity of the electrons. Therefore, uncorrelated defects like steps only have to act as a momentum source to effectively couple plasmons to the electron-hole continuum.
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页数:12
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共 43 条
[1]   Strain state analysis of hetero-epitaxial systems [J].
Al-Falou, AA ;
Kammler, M ;
Hoegen, MHV .
EUROPHYSICS LETTERS, 2005, 69 (04) :570-576
[2]   Graphitization of the 6H-SiC(0001) surface studied by HREELS [J].
Angot, T ;
Portail, M ;
Forbeaux, I ;
Layet, JM .
SURFACE SCIENCE, 2002, 502 :81-85
[3]   Strong dispersion of the surface optical phonon of silicon carbide in the near vicinity of the surface Brillouin zone center [J].
Balster, T. ;
Tautz, F. S. ;
Polyakov, V. M. ;
Ibach, H. ;
Sloboshanin, S. ;
Oettking, R. ;
Schaefer, J. A. .
SURFACE SCIENCE, 2006, 600 (14) :2886-2893
[4]   Quasiparticle dynamics in graphene [J].
Bostwick, Aaron ;
Ohta, Taisuke ;
Seyller, Thomas ;
Horn, Karsten ;
Rotenberg, Eli .
NATURE PHYSICS, 2007, 3 (01) :36-40
[5]   Defect Scattering in Graphene [J].
Chen, Jian-Hao ;
Cullen, W. G. ;
Jang, C. ;
Fuhrer, M. S. ;
Williams, E. D. .
PHYSICAL REVIEW LETTERS, 2009, 102 (23)
[6]   Surface transfer p-type doping of epitaxial graphene [J].
Chen, Wei ;
Chen, Shi ;
Qi, Dong Chen ;
Gao, Xing Yu ;
Wee, Andrew Thye Shen .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2007, 129 (34) :10418-10422
[7]   LOW-ENERGY ELECTRON-DIFFRACTION WITH ENERGY RESOLUTION [J].
CLAUS, H ;
BUSSENSCHUTT, A ;
HENZLER, M .
REVIEW OF SCIENTIFIC INSTRUMENTS, 1992, 63 (04) :2195-2199
[8]   Structural coherency of graphene on Ir(111) [J].
Coraux, Johann ;
N'Diaye, Alpha T. ;
Busse, Carsten ;
Michely, Thomas .
NANO LETTERS, 2008, 8 (02) :565-570
[9]   Interaction, growth, and ordering of epitaxial graphene on SiC{0001} surfaces: A comparative photoelectron spectroscopy study [J].
Emtsev, K. V. ;
Speck, F. ;
Seyller, Th. ;
Ley, L. ;
Riley, J. D. .
PHYSICAL REVIEW B, 2008, 77 (15)
[10]  
Emtsev KV, 2009, NAT MATER, V8, P203, DOI [10.1038/nmat2382, 10.1038/NMAT2382]