Scaling of size distributions of C60 and C70 fullerene surface islands

被引:2
|
作者
Dubrovskii, V. G. [1 ,2 ,3 ]
Berdnikov, Y. [1 ,3 ]
Olyanich, D. A. [4 ,5 ]
Mararov, V. V. [4 ,5 ]
Utas, T. V. [4 ,5 ]
Zotov, A. V. [4 ,5 ,6 ]
Saranin, A. A. [4 ,5 ]
机构
[1] St Petersburg Acad Univ, Khlopina 8-3, St Petersburg 194021, Russia
[2] RAS, Ioffe Phys Tech Inst, Politekh Skaya 26, St Petersburg 194021, Russia
[3] ITMO Univ, Kronverkskiy Pr 49, St Petersburg 197101, Russia
[4] RAS, Inst Automat & Control Proc FEB, Vladivostok 690041, Russia
[5] Far Eastern Fed Univ, Sch Nat Sci, Vladivostok 690950, Russia
[6] Vladivostok State Univ Econ & Serv, Dept Elect, Vladivostok 690600, Russia
基金
俄罗斯科学基金会;
关键词
Fullerene surface islands; Size distribution; Scaling; GROWTH; AGGREGATION; CLUSTERS;
D O I
10.1016/j.apsusc.2017.02.161
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We present experimental data and a theoretical analysis for the size distributions of C-60 and C-70 surface islands deposited onto In-modified Si(111)root 3 x root 3-Au surface under different conditions. We show that both fullerene islands feature an analytic Vicsek-Family scaling shape where the scaled size distributions are given by a power law times an incomplete beta-function with the required normalization. The power exponent in this distribution corresponds to the fractal shape of two-dimensional islands, confirmed by the experimentally observed morphologies. Quite interestingly, we do not see any significant difference between C-60 and C-70 fullerenes in terms of either scaling parameters or temperature dependence of the diffusion constants. In particular, we deduce the activation energy for surface diffusion of E-D = 140 +/- 10 meV for both types of fullerenes. (C) 2017 Elsevier B.V. All rights reserved.
引用
收藏
页码:117 / 120
页数:4
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