Iron(III) porphyrin supported on S and N co-doped graphene quantum dot as an efficient photocatalyst for aerobic oxidation of alcohols under visible light irradiation

被引：54
作者：
Mahyari, Mojtaba [1 ]
Bide, Yasamin [2 ]
Gavgani, Jaber Nasrollah [3 ]
机构：
[1] Malek Ashtar Univ Technol, Elites Adv Res Ctr, POB 16765-3454, Tehran, Iran
[2] Shahid Beheshti Univ, Fac Chem, GC, POB 19396-4716, Tehran, Iran
[3] Amirkabir Univ Technol, Dept Polymer Engn & Color Technol, POB 15875-4413, Tehran, Iran
来源：
APPLIED CATALYSIS A-GENERAL | 2016年 / 517卷
基金：
美国国家科学基金会;
关键词：
Graphene quantum dots; Photocatalyst; Aerobic oxidation; Iron(III) porphyrin; ONE-STEP SYNTHESIS; SELECTIVE OXIDATION; GOLD NANOPARTICLES; BENZYLIC ALCOHOLS; CARBON NANOTUBES; ELECTROCATALYTIC ACTIVITY; NITROGEN; CATALYSTS; WATER; GREEN;
D O I：
10.1016/j.apcata.2016.03.010
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
In this study, we report the synthesis and impressive performance of Fe(III)tetra(4-sulfonatophenyl)porphyrins (FeTSPP) supported on S and N co-doped graphene quantum dots (S, N: GQDs) as efficient, recyclable, and noble metal free heterogeneous photocatalyst for the selective aerobic oxidation of alcohols to the corresponding carbonyl compounds. It was found that FeTSPP@S, N: GQDs photocatalyst represents a novel chemical function for efficient visible light catalyzed aerobic alcohol oxidation with good conversions and selectivity in water as a green solvent at room temperature. We envision that FeTSPP@S, N: GQDs provide a promising candidate for the development of highly efficient, recyclable, and industrially applicable photocatalyst in fine chemical production with high activity. (C) 2016 Elsevier B.V. All rights reserved.
引用
收藏
页码：100 / 109
页数：10
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