CO2 capture using absorbents of mixed ionic and amine solutions

被引:6
|
作者
Yang, Jie [1 ]
Yu, Xinhai [1 ,2 ]
Yan, Jinyue [3 ,4 ]
Tu, Shan-Tung [1 ]
Xu, Maogen [1 ]
机构
[1] E China Univ Sci & Technol, Sch Mech & Power Engn, Minist Educ, Key Lab Pressure Syst & Safety, Shanghai 200237, Peoples R China
[2] E China Univ Sci & Technol, State Key Lab Bioreactor Engn, Shanghai 200237, Peoples R China
[3] Malardalen Univ, Sch Sustainable Dev Soc & Technol, Vasteras, Sweden
[4] Royal Inst Technol, Sch Chem Sci & Engn, Stockholm, Sweden
关键词
CO2; capture; amine; ionic liquid; absorbent; energy consumption; METHYLDIETHANOLAMINE; SOLUBILITY;
D O I
10.1016/j.egypro.2014.12.321
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Studies have been conducted to find new absorbents for post-combustion CO2 capture. To overcome the ILs' limits and meanwhile take their advantages, the mixed amine + IL + H2O solutions as CO2 capture absorbent were investigated in a CO2 absorption/desorption loop setup. It was found that with an increase in IL concentration, the viscosity of the mixed solution rose while the energy required for absorbent regeneration decreased. In addition, no IL loss was detected and the amine loss per ton of captured CO2 was considerably lower than that of aqueous amine solution. The viscosity of the best candidate of 30 wt% MEA + 40 wt% [bmim][BF4] + 30 wt% H2O is close to the value of aqueous amine solution, indicating that the ionic liquid disadvantage of high viscosity can be overcome for absorbent delivery of CO2 capture. (C) 2014 The Authors. Published by Elsevier Ltd. This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/3.0/).
引用
收藏
页码:2849 / 2853
页数:5
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